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A possible pathway for rapid growth of sulfate during haze days in China
Li, Guohui1; Bei, Naifang2; Cao, Junji1; Huang, Rujin1; Wu, Jiarui1; Feng, Tian1,2; Wang, Yichen1; Liu, Suixin1; Zhang, Qiang3; Tie, Xuexi1; Molina, Luisa T.4,5
2017-03-07
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
卷号17期号:5页码:3301-3316
文章类型Article
摘要Rapid industrialization and urbanization have caused frequent occurrence of haze in China during wintertime in recent years. The sulfate aerosol is one of the most important components of fine particles (PM2.5) in the atmosphere, contributing significantly to the haze formation. However, the heterogeneous formation mechanism of sulfate remains poorly characterized. The relationships of the observed sulfate with PM2.5, iron, and relative humidity in Xi'an, China have been employed to evaluate the mechanism and to develop a parameterization of the sulfate heterogeneous formation involving aerosol water for incorporation into atmospheric chemical transport models. Model simulations with the proposed parameterization can successfully reproduce the observed sulfate rapid growth and diurnal variations in Xi'an and Beijing, China. Reasonable representation of sulfate heterogeneous formation in chemical transport models considerably improves the PM2.5 simulations, providing the underlying basis for better understanding the haze formation and supporting the design and implementation of emission control strategies.
WOS标题词Science & Technology ; Physical Sciences
DOI10.5194/acp-17-3301-2017
关键词[WOS]MEXICO-CITY ; MCMA-2006/MILAGRO CAMPAIGN ; HETEROGENEOUS REACTIONS ; PARTICULATE MATTER ; INORGANIC AEROSOLS ; ACID DEPOSITION ; URBAN FOG ; MODEL ; SO2 ; PHOTOCHEMISTRY
收录类别SCI
语种英语
WOS研究方向Meteorology & Atmospheric Sciences
WOS类目Meteorology & Atmospheric Sciences
WOS记录号WOS:000396128600003
引用统计
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/5496
专题粉尘与环境研究室
作者单位1.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Key Lab Aerosol Chem & Phys, Xian, Peoples R China
2.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Shaanxi, Peoples R China
3.Tsinghua Univ, Dept Earth Syst Sci, Beijing, Peoples R China
4.Molina Ctr Energy & Environm, La Jolla, CA USA
5.MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA
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Li, Guohui,Bei, Naifang,Cao, Junji,et al. A possible pathway for rapid growth of sulfate during haze days in China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(5):3301-3316.
APA Li, Guohui.,Bei, Naifang.,Cao, Junji.,Huang, Rujin.,Wu, Jiarui.,...&Molina, Luisa T..(2017).A possible pathway for rapid growth of sulfate during haze days in China.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(5),3301-3316.
MLA Li, Guohui,et al."A possible pathway for rapid growth of sulfate during haze days in China".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.5(2017):3301-3316.
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