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Seasonal and diurnal variations of mono- and di-carbonyls in Xi'an, China
Dai, WT (Dai, W. T.)[1]; Ho, SSH (Ho, Steven Sai Hang)[1,2]; Ho, KF (Ho, K. F.)[1,3]; Liu, WD (Liu, W. D.)[4]; Cao, JJ (Cao, J. J.)[1]; Lee, SC (Lee, S. C.)[4]
2012-09-30
发表期刊ATMOSPHERIC RESEARCH
卷号113页码:102-112
文章类型期刊论文
摘要

Seventeen carbonyls in urban ambient air were quantified in summer (June 2009) and winter (January 2010) in an urban site located in Xi'an, China. Formaldehyde, acetaldehyde and acetone were the three most abundant carbonyls in the atmosphere with the concentrations of 6.54 +/- 2.38 ppbv, 2.08 +/- 1.07 ppbv and 2.74 +/- 1.14 ppbv in summer (from 14th to 24th June, 2009), respectively. In winter, the concentrations were 4.46 +/- 1.74 ppbv, 6.52 +/- 3.88 ppbv and 3.87 +/- 2.33 ppbv respectively from 4th January, 2010 to 10th January, 2010. Most carbonyls had higher concentrations in winter than in summer. And majority of the species had higher concentrations in daytime than in nighttime, indicating photochemical oxidation/human activities played an important role in diurnal variation. Formaldehyde/acetaldehyde ratios (F/A) in summer (2.14) was much higher than that in winter (0.47), showing significant effect of photochemical oxidation in the urban air during summer. Acetaldehyde/propionaldehyde (A/P) average ratio was 12.2 in wintertime, implying anthropogenic emission was the major source of carbonyls in Xi'an. In addition, the ratio of acetone to methylglyoxal (A/M) is used to determine the impact of photochemistry in the atmosphere. The average acetone/methylglyoxal ratio (10.3 +/- 2.3) in summer was lower than that in winter (21.3 +/- 5.1) in Xi'an. Strong correlations among some carbonyls imply that they came from the same pollution sources. Formaldehyde and acetaldehyde play a very important role in photochemical smog formation. Methylglyoxal and glyoxal also have significant contribution to ozone formation potential.

关键词Carbonyl Compounds Seasonal And Diurnal Variations Correlation Xi'an
DOI10.1016/j.atmosres.2012.05.001
收录类别SCI ; EI
语种英语
引用统计
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/10088
专题粉尘与环境研究室
通讯作者Ho, KF (Ho, K. F.)[1,3]
作者单位1.SKLLQG, Institute of Earth Environment Chinese Academy of Sciences, Xi'an 710075, China;
2.Division of Atmospheric Sciences, Desert Research Institute, Reno, NV 89512, United States;
3.School of Public Health and Primary Care, The Chinese University of Hong Kong, Shatin, Hong Kong, China;
4.Research Center of Urban Environmental Technology and Management, Department of Civil and Structural Engineering, The Hong Kong Polytechnic University,Hung Hom, Kowloon, Hong Kong, China
推荐引用方式
GB/T 7714
Dai, WT ,Ho, SSH ,Ho, KF ,et al. Seasonal and diurnal variations of mono- and di-carbonyls in Xi'an, China[J]. ATMOSPHERIC RESEARCH,2012,113:102-112.
APA Dai, WT ,Ho, SSH ,Ho, KF ,Liu, WD ,Cao, JJ ,&Lee, SC .(2012).Seasonal and diurnal variations of mono- and di-carbonyls in Xi'an, China.ATMOSPHERIC RESEARCH,113,102-112.
MLA Dai, WT ,et al."Seasonal and diurnal variations of mono- and di-carbonyls in Xi'an, China".ATMOSPHERIC RESEARCH 113(2012):102-112.
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