Speciation and migration of 129I in soil profiles | |
Luo, MY (Luo, Maoyi)[ 3 ]; Hou, XL (Hou, Xiaolin)[ 1,2,4 ]; Zhou, WJ (Zhou, Weijian)[ 1,2 ]; He, CH (He, Chaohui)[ 3 ]; Chen, N (Chen, Ning)[ 1,2 ]; Liu, Q (Liu, Qi)[ 1,2 ]; Zhang, LY (Zhang, Luoyuan)[ 1,2,4 ] | |
2013-04-01 | |
发表期刊 | Journal of Environmental Radioactivity |
卷号 | 118页码:30-39 |
文章类型 | 期刊论文 |
摘要 | A method has been developed for speciation analysis of ultra low level I-129 in soil using sequential extraction combined with coprecipitation for separation of carrier free iodine and AMS measurement of I-129. Two loess profiles collected from northwest China were analyzed for species of I-129 and I-127. Similar partitioning of I-129 and I-122 was observed in the loess profiles, the distribution of iodine isotopes followed an order of organic > leachable > reducible > residue. The I-129 concentrations and I-129/I-127 ratios decreased exponentially with the depth, and 2 orders of magnitude lower in the deepest layer (60 and 90 cm) compared with the top layer, indicating a significant contribution of anthropogenic input in the upper layer, and high retention of I-129 in soil. The mobility of I-129 in different fractions decreased in an order of leachable > organic > oxides > residue. The results suggest that migration of iodine downwards in the soil profile is a slow process; the oxides and residue are the less mobile fractions of iodine. |
关键词 | Iodine-129 Fractionation Ams Speciation Analysis Loess Mobility |
DOI | 10.1016/j.atmosenv.2013.07.024 |
收录类别 | SCI ; EI |
语种 | 英语 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ieecas.cn/handle/361006/9973 |
专题 | 加速器质谱中心 |
通讯作者 | Hou, XL (Hou, Xiaolin)[ 1,2,4 ] |
作者单位 | 1.Xi’an AMS Center and KLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710075, China; 2.School of Nuclear Science and Technology, Xi’an Jiaotong University, Xi’an 710049, China; 3.Center for Nuclear Technologies, Technical University of Denmark, Risø Campus, DK-4000 Roskilde, Denmark |
推荐引用方式 GB/T 7714 | Luo, MY ,Hou, XL ,Zhou, WJ ,et al. Speciation and migration of 129I in soil profiles[J]. Journal of Environmental Radioactivity,2013,118:30-39. |
APA | Luo, MY .,Hou, XL .,Zhou, WJ .,He, CH .,Chen, N .,...&Zhang, LY .(2013).Speciation and migration of 129I in soil profiles.Journal of Environmental Radioactivity,118,30-39. |
MLA | Luo, MY ,et al."Speciation and migration of 129I in soil profiles".Journal of Environmental Radioactivity 118(2013):30-39. |
条目包含的文件 | ||||||
文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | ||
Speciation and migra(1234KB) | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | 请求全文 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论