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Diurnal and seasonal trends of carbonyl compounds in roadside, urban, and suburban environment of Hong Kong
Cheng, Y (Cheng, Y.)[ 1,2 ]; Lee, SC (Lee, S. C.)[ 3 ]; Huang, Y (Huang, Y.)[ 3 ]; Ho, KF (Ho, K. F.)[ 4 ]; Ho, SSH (Ho, S. S. H.)[ 2,4,5 ]; Yau, PS (Yau, P. S.)[ 3 ]; Louie, PKK (Louie, P. K. K.)[ 6 ]; Zhang, RJ (Zhang, R. J.)[ 7 ]
2014-06-01
发表期刊ATMOSPHERIC ENVIRONMENT
卷号89页码:43-51
文章类型期刊论文
摘要

Seasonal and diurnal variations of carbonyl compounds were investigated in roadside (MK), urban (TW), and suburban (UST) environments in Hong Kong. Thirteen carbonyls (C1-C6) were identified and quantified in the samples. The average total quantified carbonyl concentrations decreased in the order of roadside (12.16 +/- 3.52 mu g m(-3)), urban (10.45 +/- 4.82 mu g m(-3)), and suburban (5.14 +/- 3.35 mu g m(-3)). Formaldehyde was the most abundant species, accounting for similar to 52%, similar to 52%, and similar to 46% of total measured carbonyls at MK, TW, and UST, respectively. At MK, the summer/winter ratios of most carbonyls were below one. The diurnal variations were associated with traffic flows, with high concentrations in daytime but low in nighttime. Good correlations were found between most carbonyls and carbon monoxide (CO), showing primary vehicular emission was the major source at the roadside location. In contrast, the summer/winter ratios of most carbonyls were larger than one at the urban site of TW and their carbonyls correlated well with secondary pollutant of ozone (O-3), indicating photochemical reactions contributed significantly in the formation of carbonyls, especially in summer. Distinct diurnal variations of carbonyls were observed at TW on a hazy winter day of 28 Jan 2012. Most carbonyl concentrations reached the first peak at noontime and had the second peak in the evening. The first peak was ascribed to be the products of photochemical reactions as maximum concentrations of nitrogen monoxide (NO) and O-3 occurred just before and after the carbonyl peak, respectively. The correlations among the carbonyl species were strong in summer but fair in winter at UST. Natural sources (e.g. biogenic) were usually the major source at the suburban, as far as its surrounding environment is concerned.

关键词Carbonyls Diurnal Variations Seasonal Variations
DOI10.1016/j.atmosenv.2014.02.014
收录类别SCI ; EI
语种英语
引用统计
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/9695
专题粉尘与环境研究室
通讯作者Cheng, Y (Cheng, Y.)[ 1,2 ]
作者单位1.Department of Environmental Science and Technology, School of Human Settlements and Civil Engineering, Xi’an Jiaotong University, No. 28 XianningWest Road, Xi’an, Shaanxi 710049, China;
2.SKLLQG, Institute of Earth and Environment, CAS, Xi’an, Shaanxi 710075, China;
3.Department of Civil and Environmental Engineering, Research Center for Environmental Technology and Management, The Hong Kong PolytechnicUniversity, Hung Hom, Kowloon, Hong Kong;
4.Jockey Club School of Public Health and Primary Care, The Chinese University of Hong Kong, Hong Kong, China;
5.Division of Atmospheric Sciences, Desert Research Institute, 2215 Raggio Pathway, Reno, NV 89512, United States;
6.Hong Kong Environmental Protection Department, 47/F, Revenue Tower, 5 Gloucester Road, Wan Chai, Hong Kong, China;
7.Key Laboratory of Regional Climate-Environment Research for Temperate East Asia, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing100029, China
推荐引用方式
GB/T 7714
Cheng, Y ,Lee, SC ,Huang, Y ,et al. Diurnal and seasonal trends of carbonyl compounds in roadside, urban, and suburban environment of Hong Kong[J]. ATMOSPHERIC ENVIRONMENT,2014,89:43-51.
APA Cheng, Y .,Lee, SC .,Huang, Y .,Ho, KF .,Ho, SSH .,...&Zhang, RJ .(2014).Diurnal and seasonal trends of carbonyl compounds in roadside, urban, and suburban environment of Hong Kong.ATMOSPHERIC ENVIRONMENT,89,43-51.
MLA Cheng, Y ,et al."Diurnal and seasonal trends of carbonyl compounds in roadside, urban, and suburban environment of Hong Kong".ATMOSPHERIC ENVIRONMENT 89(2014):43-51.
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