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Iodine-129 in Snow and Seawater in the Antarctic: Level and Source
Xing,S(Xing,Shan)[1,5]; Hou,XL(Hou,Xiaolin)[1,2]; Aldahan,A(Aldahan,Ala)[3,6]; Possnert,G(Possnert,Göran)[4]; Shi,KL(Shi,Keliang)[2,7]; Yi,P(Yi,Peng)[3,8]; Zhou,WJ(Zhou,Weijian)[1]
2015-05-05
发表期刊Environmental Science & Technology
卷号49期号:11页码:6691-6700
文章类型期刊论文
摘要

Anthropogenic 129I has been released to the environment in different ways and chemical species by human nuclear activities since the 1940s. These sources provide ideal tools to trace the dispersion of volatile pollutants in the atmosphere. Snow and seawater samples collected in Bellingshausen, Amundsen, and Ross Seas in Antarctica in 2011 were analyzed for 129I and 127I, including organic forms; it was observed that 129I/127I atomic ratios in the Antarctic surface seawater ((6.1−13) × 10−12) are about 2 orders of magnitude lower than those in the Antarctic snow ((6.8−9.5) × 10−10), but 4−6 times higher than the prenuclear level (1.5 × 10−12), indicating a predominantly anthropogenic source of 129I in the Antarctic environment. The 129I level in snow in Antarctica is 2−4 orders of magnitude lower than that in the Northern Hemisphere, but is not significantly higher than that observed in other sites in the Southern Hemisphere. This feature indicates that 129I in Antarctic snow mainly originates from atmospheric nuclear weapons testing from 1945 to 1980; resuspension and re-emission of the fallout 129I in the Southern Hemisphere maintains the 129I level in the Antarctic atmosphere. 129I directly released to the atmosphere and re-emitted marine discharged 129I from reprocessing plants in Europe might not significantly disperse to Antarctica.

DOI10.1021/acs.est.5b01234
收录类别SCI
语种英语
引用统计
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/9481
专题加速器质谱中心
作者单位1.Xi’an AMS Center, SKLLQG, Shaanxi Key Laboratory of Accelerator Mass Spectrometry Technology and Application, Institute ofEarth Environment, CAS, Xi’an 710061, China;
2.Technical University of Denmark, Center for Nuclear Technologies, Risø Campus, Roskilde 4000, Denmark;
3.Department of Geology, United Arab Emirates University, Al Ain, United Arab Emirates;
4.Tandem Laboratory, Uppsala University, Uppsala 75120, Sweden;
5.University of Chinese Academy of Science, Beijing 100049, China;
6.Department of Earth Sciences, Uppsala University, Uppsala 75120, Sweden;
7.School of Nuclear Science and Technology, Lanzhou University, 73000, Lanzhou, China;
8.College of Hydrology & Water Resources, Hohai University, 210098, Nanjing, China
推荐引用方式
GB/T 7714
Xing,S,Hou,XL,Aldahan,A,et al. Iodine-129 in Snow and Seawater in the Antarctic: Level and Source[J]. Environmental Science & Technology,2015,49(11):6691-6700.
APA Xing,S.,Hou,XL.,Aldahan,A.,Possnert,G.,Shi,KL.,...&Zhou,WJ.(2015).Iodine-129 in Snow and Seawater in the Antarctic: Level and Source.Environmental Science & Technology,49(11),6691-6700.
MLA Xing,S,et al."Iodine-129 in Snow and Seawater in the Antarctic: Level and Source".Environmental Science & Technology 49.11(2015):6691-6700.
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