Facile synthesis of porous graphene-like carbon nitride (C6N9H3) withexcellent photocatalytic activity for NO removal
Dong,GH(Dong,Guohui)[1,2]; Ho,WK(Ho,Wingkei)[1,3]; Li,YH(Li,Yuhan)[1]; Zhang,LZ(Zhang,Lizhi)[2]
2015-03
发表期刊Applied Catalysis B: Environmental
卷号174-175期号:2015页码:477-485
文章类型期刊论文
摘要

We reported the possible synthesis of a new porous graphene-like carbon nitride (C6N9H3) by simply adding hydrochloric acid in the precursor of block g-C3N4. The formation of the porous graphene-like C6N9H3 can be attributed to the change in the thermal condensation modal of the precursor and the acidic condition induced by Cl− and H+. The photocatalytic activity of the samples was evaluated by the removal of NO under visible light illumination. We found that the porous graphene-like C6N9H3 exhibited enhanced photocatalytic activity compared to the block g-C3N4.We also researched the removal mechanism and found that the removal of NO in our systems was due to the synergic effect of h+ and •O2−. This study could shed light on the design of efficient photocatalysts and facilitate a deep understanding of the NO removal mechanism through photocatalytic technology.

关键词Porous C6n9h3 Photocatalytic No Removal Visible Light
DOI10.1016/j.apcatb.2015.03.035
收录类别SCI
语种英语
引用统计
被引频次:161[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/9465
专题黄土与第四纪地质国家重点实验室(2010~)
作者单位1.Department of Science and Environmental Studies and Centre for Education in Environmental Sustainability, The Hong Kong Institute of Education, Tai Po,N.T. Hong Kong, People’s Republic of China;
2.Key Laboratory of Pesticide and Chemical Biology of Ministry of Education, College of Chemistry, Central China Normal University, Wuhan 430079,People’s Republic of China;
3.Key Lab of Aerosol Chemistry & Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710075, China
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Dong,GH,Ho,WK,Li,YH,et al. Facile synthesis of porous graphene-like carbon nitride (C6N9H3) withexcellent photocatalytic activity for NO removal[J]. Applied Catalysis B: Environmental,2015,174-175(2015):477-485.
APA Dong,GH,Ho,WK,Li,YH,&Zhang,LZ.(2015).Facile synthesis of porous graphene-like carbon nitride (C6N9H3) withexcellent photocatalytic activity for NO removal.Applied Catalysis B: Environmental,174-175(2015),477-485.
MLA Dong,GH,et al."Facile synthesis of porous graphene-like carbon nitride (C6N9H3) withexcellent photocatalytic activity for NO removal".Applied Catalysis B: Environmental 174-175.2015(2015):477-485.
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