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Airborne particulate endocrine disrupting compounds in China:Compositions, size distributions and seasonal variations ofphthalate esters and bisphenol A
Li,JJ(Li,Jianjun)[1]; Wang,GH(Wang,Gehui)[1]
2015
发表期刊Atmospheric Research
卷号154期号:2015页码:138-145
文章类型期刊论文
摘要

Phthalate esters and bisphenol A (BPA) are endocrine disrupting compounds (EDCs) and ubiquitously occur in the environment. In the past decade we have characterized atmospheric organic aerosols from various environments (e.g., urban, rural, mountain and marine) of East Asia on a molecular level, but not investigated EDCs in the samples. In the current study we re-analyzed our database for concentrations, compositions and size distributions of phthalates and BPA and compared with those in the literature to improve the understanding on air pollution status in China. Our results showed that airborne particulate phthalates and BPA are 63–1162 ng m−3 and 1.0–20 ng m−3 in the urban regions in China, respectively, being one to two orders of magnitude higher than those in the developed countries. Among the detected phthalates in Chinese urban areas, bis(2-ethylhexyl) phthalate (BEHP) is the predominant congener, contributing to 23–79% (ave. 53 ± 15%) of the total phthalates. Concentrations of phthalates and bisphenol A in Shanghai and Xi'an (two mega-cities in China) in 2009 were 3–84% lower than those in 2003, probably indicating a positive effect of the government's air pollution control in the recent years. Phthalates are higher in summer than in winter, because they are not chemically bonded to the polymeric matrix and more easily evaporate into the air under higher temperature conditions. Based on the size distribution observation, we found that diisobutyl and dibutyl phthalates mainly exist in coarse particles because of high volatilities, in contrast to BEHP and BPA, which are dominant in fine particles due to less volatility. Our results also indicate that BPA is mostly derived from the open burning of solid waste while phthalates are derived from both direct evaporation from the matrix and solid waste combustion.

关键词Phthalate Esters Bisphenol a Bis(2-ethylhexyl) Phthalate (Behp) Endocrine Disrupting Compounds (Edcs) Open Burning Of Solid Waste
DOI10.1016/j.atmosres.2014.11.013
收录类别SCI
语种英语
引用统计
被引频次:31[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/9431
专题粉尘与环境研究室
作者单位State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710075, China
第一作者单位黄土与第四纪地质国家重点实验室(1985-2004)
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Li,JJ,Wang,GH. Airborne particulate endocrine disrupting compounds in China:Compositions, size distributions and seasonal variations ofphthalate esters and bisphenol A[J]. Atmospheric Research,2015,154(2015):138-145.
APA Li,JJ,&Wang,GH.(2015).Airborne particulate endocrine disrupting compounds in China:Compositions, size distributions and seasonal variations ofphthalate esters and bisphenol A.Atmospheric Research,154(2015),138-145.
MLA Li,JJ,et al."Airborne particulate endocrine disrupting compounds in China:Compositions, size distributions and seasonal variations ofphthalate esters and bisphenol A".Atmospheric Research 154.2015(2015):138-145.
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