Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow

doi:10.1016/j.chemosphere.2016.03.069

IEECAS OpenIR > 黄土与第四纪地质国家重点实验室（2010~）

	Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow
	Zhao, Yan 1; Zhang, Yingyi 1; Fu, Pingqing 2; Ho, Steven Sai Hang 3,4; Ho, Kin Fai 5; Liu, Fobang 6; Zou, Shichun 7; Wang, Shan 1; Lai, Senchao 1,6
	2016-06-01
发表期刊	CHEMOSPHERE
卷号	153 期号:2016 页码:332-339
文章类型	Article
摘要	Filter samples of total suspended particle (TSP) collected during a cruise campaign over the northern South China Sea (SCS) from September to October 2013 were analyzed for non-polar organic compounds (NPOCs) as well as organic carbon (OC), elemental carbon (EC) and water-soluble ions. A total of 115 NPOCs species in groups of n-alkanes, polycyclic aromatic hydrocarbons (PAHs), iso-/antiso-alkanes, hopanes, steranes, methylalkanes, branched alkanes, cycloalkanes, alkenes and phthalates were detected. The characteristics of NPOCs in marine TSP samples were investigated to understand the sources from the Asian continent and other regions. The concentrations of total NPOCs ranged from 19.8 to 288.2 ng/m(3) with an average of 87.9 ng/m(3), which accounted for 0.8-1.7% (average 1.0%) of organic matter (OM). n-Alkanes was the predominant group, accounting for 43.1-79.5%, followed by PAHs (5.5-44.4%) and hopanes (1.6-11.4%). We found that primary combustion (biomass burning/fossil fuel combustion) was the dominant source for the majority of NPOCs (89.1%). Biomass burning in southern/southeastern China via long-range transport was proposed to be a major contributor of NPOCs in marine aerosols over the northern SCS, suggested by the significant correlations between nss-K+ and NPOCs groups as well as the analysis of air mass back-trajectory and fire spots. For the samples with strong continental influence, the strong enhancement in concentrations of n-alkanes, PAHs, hopanes and steranes were attributed to fossil fuel (coal/petroleum) combustion. In addition, terrestrial plants waxes were another contributor to NPOCs. (C) 2016 Elsevier Ltd. All rights reserved.
关键词	Northern South China Sea N-alkanes Pahs Hopanes Biomass Burning Long-range Transport
WOS标题词	Science & Technology ; Life Sciences & Biomedicine
DOI	10.1016/j.chemosphere.2016.03.069
关键词[WOS]	ATMOSPHERIC PARTICULATE MATTER ; MOLECULAR MARKER ; PACIFIC-OCEAN ; HONG-KONG ; TRACERS ; PAHS ; IDENTIFICATION ; TROPOSPHERE ; COMBUSTION ; DEPOSITION
收录类别	SCI
语种	英语
WOS研究方向	Environmental Sciences & Ecology
WOS类目	Environmental Sciences
WOS记录号	WOS:000375628800039
引用统计	被引频次：25[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.ieecas.cn/handle/361006/5786
专题	黄土与第四纪地质国家重点实验室（2010~）
作者单位	1.S China Univ Technol, Sch Environm & Energy, Guangdong Prov Key Lab Atmospher Environm & Pollu, Guangzhou 510641, Guangdong, Peoples R China 2.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China 3.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Peoples R China 4.Univ Nevada, Desert Res Inst, Div Atmospher Sci, 2215 Raggio Pathway, Reno, NV 89506 USA 5.Chinese Univ Hong Kong, Jockey Club Sch Publ Hlth & Primary Care, Shatin, Hong Kong, Peoples R China 6.Max Planck Inst Chem, Multiphase Chem Dept, Mainz, Germany 7.Sun Yat Sen Univ, Sch Marine Sci, Guangzhou 510275, Guangdong, Peoples R China
推荐引用方式 GB/T 7714	Zhao, Yan,Zhang, Yingyi,Fu, Pingqing,et al. Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow[J]. CHEMOSPHERE,2016,153(2016):332-339.
APA	Zhao, Yan.,Zhang, Yingyi.,Fu, Pingqing.,Ho, Steven Sai Hang.,Ho, Kin Fai.,...&Lai, Senchao.(2016).Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow.CHEMOSPHERE,153(2016),332-339.
MLA	Zhao, Yan,et al."Non-polar organic compounds in marine aerosols over the northern South China Sea: Influence of continental outflow".CHEMOSPHERE 153.2016(2016):332-339.

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