Occurrence and levels of polybrominated diphenyl ethers in surface sediments from the Yellow River Estuary, China
Yuan, Zijiao1,2,3,4; Liu, Guijian1,2,3; Lam, Michael Hon Wah3,4; Liu, Houqi1; Da, Chunnian1
2016-05-01
发表期刊ENVIRONMENTAL POLLUTION
卷号212期号:2016页码:147-154
文章类型Article
摘要A total of 21 surface sediments collected from the Yellow River Estuary, China were analyzed for 40 kinds of polybrominated diphenyl ethers (PBDEs) using gas chromatography-mass spectrometry (GC-MS). Their levels, spatial distribution, congener profiles and possible sources were investigated. Only ten congeners were detected in the sediments. The total concentrations of the lower brominated BDEs (Sigma PBDEslow, PBDEs excluding BDE 209) and BDE 209 ranged from 0.482 ng/g to 1.07 ng/g and 1.16-5.40 ng/g, with an average value of 0.690 and 2.79 ng/g, respectively, which were both at the low end of the global contamination level. The congener profiles were dominated by BDE 209, with the average value accounting for 79.2% of the total PBDEs in the sediment samples. Among the nine lower brominated BDE congeners, BDE 47, 99 and 183 had high abundances. Although the commercial Penta/Octa-BDE products have been banned in most countries, the residual commercial Penta/Octa/Deca-BDE products and the debromination of highly brominated BDE compounds such as BDE 209 were still found to be the possible sources for the trace level of PBDEs in the present study area. In spite of the gradual removal of the commercial PBDEs in the world, the present research results further suggested that scientific attention should not be reduced on the issue of environmental contamination caused by these outdated chemical compounds. (C) 2016 Elsevier Ltd. All rights reserved.
关键词Yellow River Polybrominated Diphenyl Ethers Surface Sediments Congener Profiles Possible Sources
WOS标题词Science & Technology ; Life Sciences & Biomedicine
DOI10.1016/j.envpol.2016.01.058
关键词[WOS]POLYCYCLIC AROMATIC-HYDROCARBONS ; POLYCHLORINATED-BIPHENYLS PCBS ; BROMINATED FLAME RETARDANTS ; STARLINGS STURNUS-VULGARIS ; OIL-FIELD CITY ; HUMAN EXPOSURE ; SOUTH CHINA ; NORTH CHINA ; SPATIAL-DISTRIBUTION ; BUILDING SURFACES
收录类别SCI
语种英语
WOS研究方向Environmental Sciences & Ecology
WOS类目Environmental Sciences
WOS记录号WOS:000376800000019
引用统计
被引频次:35[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/5734
专题黄土与第四纪地质国家重点实验室(2010~)
作者单位1.Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China
2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710075, Shaanxi, Peoples R China
3.Univ Sci & Technol China City Univ Hong Kong Join, Suzhou 215123, Jiangsu, Peoples R China
4.City Univ Hong Kong, Dept Biol & Chem, Tat Chee Ave, Hong Kong, Hong Kong, Peoples R China
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Yuan, Zijiao,Liu, Guijian,Lam, Michael Hon Wah,et al. Occurrence and levels of polybrominated diphenyl ethers in surface sediments from the Yellow River Estuary, China[J]. ENVIRONMENTAL POLLUTION,2016,212(2016):147-154.
APA Yuan, Zijiao,Liu, Guijian,Lam, Michael Hon Wah,Liu, Houqi,&Da, Chunnian.(2016).Occurrence and levels of polybrominated diphenyl ethers in surface sediments from the Yellow River Estuary, China.ENVIRONMENTAL POLLUTION,212(2016),147-154.
MLA Yuan, Zijiao,et al."Occurrence and levels of polybrominated diphenyl ethers in surface sediments from the Yellow River Estuary, China".ENVIRONMENTAL POLLUTION 212.2016(2016):147-154.
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