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High Selectivity of Visible-Light-Driven La-doped TiO2 Photocatalysts for NORemoval
Huang,Y(Huang,Yu)1; Cao,JJ(Cao,Junji)1; Kang,F(Kang,Fei)2; You,SJ(You,Shengjie)2; Chang,CW(Chang,Chia-Wei)2; Wang,YF(Wang,Yafen)2; Wang,Yafen
2017-10
发表期刊Aerosol and Air Quality Research
卷号17期号:10页码:2555-2565
文章类型期刊论文
摘要Semiconductors mediated by rare earth metals (REMs) have attracted attention with regard to the degradation of pollutants. In order to enhance the visible response of TiO2, La-doped TiO2 (La-TO) photocatalysts with visible-light-driven capacity for NO removal were successfully synthesized in this study via a facile sol-gel method followed by calcination. A series of La-TiO2 samples with differing weight ratios were evaluated for their photocatalytic performances. It was found that 3% La integrated with TiO2 (in mass ratio) could enhance the removal efficiency of NO (up to 32%) under solar light, which is more than twice that seen with pure TiO2. The resulting products were characterized by a series of techniques, such as XRD, FTIR, UV-vis DRS, BET and (photo)electrochemical analysis. The results indicated that La-doped TiO2 can harvest visible light due to the relatively narrow band gap (from 2.98 to 2.75 eV). More importantly, La dopant improved electron-hole separation and suppressed charge carrier recombination, due to the synergistic effect. Furthermore, La-doped TiO2 increased the photo-oxidation efficiency of the transformation from NO to NO3–, owing to inhibition of the production of intermediate NO2 (0.02%). To the best of our knowledge, this study is the first time that La-doped TiO2 has been used to eliminate NO (at the ppb level) in the atmosphere. This study provides a facile and controllable route to fabricate La-TO photocatalyst for NO abatement with high selectivity of NO2 under visible light.
关键词La-doped Tio2 Photocatalysis No Removal
DOI10.4209/aaqr.2017.08.0282
收录类别SCI
所属项目编号EPA-105-XB05 ; 41401567 ; 41573138
语种英语
项目资助者Environmental Protection Administration Executive Yuan,Taiwan ; Environmental Protection Administration Executive Yuan,Taiwan ; National Science Foundation of China ; National Science Foundation of China
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/5598
专题粉尘与环境研究室
通讯作者Wang,Yafen
作者单位1.Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an710061, China
2.Department of Environmental Engineering, Chung Yuan Christian University, Taoyuan 32023, Taiwan
推荐引用方式
GB/T 7714
Huang,Y,Cao,JJ,Kang,F,et al. High Selectivity of Visible-Light-Driven La-doped TiO2 Photocatalysts for NORemoval[J]. Aerosol and Air Quality Research,2017,17(10):2555-2565.
APA Huang,Y.,Cao,JJ.,Kang,F.,You,SJ.,Chang,CW.,...&Wang,Yafen.(2017).High Selectivity of Visible-Light-Driven La-doped TiO2 Photocatalysts for NORemoval.Aerosol and Air Quality Research,17(10),2555-2565.
MLA Huang,Y,et al."High Selectivity of Visible-Light-Driven La-doped TiO2 Photocatalysts for NORemoval".Aerosol and Air Quality Research 17.10(2017):2555-2565.
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