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Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland
Lin, Chunshui1,2,3,4; Ceburnis, Darius1,2; Hellebust, Stig5,6; Buckley, Paul5,6; Wenger, John5,6; Canonaco, Francesco7; Prevot, Andre Stephan Henry7; Huang, Ru-Jin1,2,3,4,7; O'Dowd, Colin1,2; Ovadnevaite, Jurgita1,2
2017-09-19
发表期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
卷号51期号:18页码:10624-10632
文章类型Article
摘要An aerosol chemical speciation monitor (ACSM) was deployed to study the primary nonrefractory submicron particulate matter emissions from the burning of commercially available solid fuels (peat, coal, and wood) typically used in European domestic fuel stoves. Organic mass spectra (MS) from burning wood, peat, and coal were characterized and intercompared for factor analysis against ambient data. The reference profiles characterized in this study were used to estimate the contribution of solid fuel sources, along with oil combustion, to ambient pollution in Galway, Ireland using the multilinear engine (ME-2). During periods influenced by marine air masses, local source contribution had dominant impact and nonsea-spray primary organic emissions comprised 88% of total organic aerosol mass, with peat burning found to be the greatest contributor (39%), followed by oil (21%), coal (17%), and wood (11%). In contrast, the resolved oxygenated organic aerosol (OOA) dominated the aerosol composition in continental air masses, with contributions of 50%, compared to 12% in marine air masses. The source apportionment results suggest that the use of domestic solid fuels (peat, wood, and coal) for home heating is the major source of evening and night-time particulate pollution events despite their small use.
WOS标题词Science & Technology ; Technology ; Life Sciences & Biomedicine
DOI10.1021/acs.est.7b01926
关键词[WOS]POSITIVE MATRIX FACTORIZATION ; MASS-SPECTROMETER DATA ; SOURCE APPORTIONMENT ; AIR-POLLUTION ; CHEMICAL-COMPOSITION ; CORK HARBOR ; COMBUSTION ; EMISSIONS ; COMPONENTS ; PARTICLES
收录类别SCI
语种英语
WOS研究方向Engineering ; Environmental Sciences & Ecology
WOS类目Engineering, Environmental ; Environmental Sciences
WOS记录号WOS:000411549800040
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/5413
专题粉尘与环境研究室
作者单位1.Natl Univ Ireland Galway, Sch Phys, Univ Rd, Galway H91CF50, Ireland
2.Natl Univ Ireland Galway, Ryan Inst, Ctr Climate & Air Pollut Studies, Univ Rd, Galway H91CF50, Ireland
3.Chinese Acad Sci, State Key Lab Loess & Quaternary Geol, Inst Earth Environm, Xian 710061, Shaanxi, Peoples R China
4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China
5.Univ Coll Cork, Dept Chem, Cork T23XE10, Ireland
6.Univ Coll Cork, Environm Res Inst, Cork T23XE10, Ireland
7.Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland
推荐引用方式
GB/T 7714
Lin, Chunshui,Ceburnis, Darius,Hellebust, Stig,et al. Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2017,51(18):10624-10632.
APA Lin, Chunshui.,Ceburnis, Darius.,Hellebust, Stig.,Buckley, Paul.,Wenger, John.,...&Ovadnevaite, Jurgita.(2017).Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland.ENVIRONMENTAL SCIENCE & TECHNOLOGY,51(18),10624-10632.
MLA Lin, Chunshui,et al."Characterization of Primary Organic Aerosol from Domestic Wood, Peat, and Coal Burning in Ireland".ENVIRONMENTAL SCIENCE & TECHNOLOGY 51.18(2017):10624-10632.
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