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Sources and physicochemical characteristics of blackcarbon aerosol from the southeastern Tibetan Plateau:internal mixing enhances light absorption
Wang,QY(Wang,Qiyuan)1; Cao,JJ(Cao,Junji)1,2; Han,YM(Han,Yongming)1,3; Tian,J(Tian,Jie)4; Zhu,CS(Zhu,Chongshu)1; Zhang,YG(Zhang,Yonggang)1; Zhang,NN(Zhang,Ningning)1; Shen,ZX(Shen,Zhenxing)4; Ni,HY(Ni,Haiyan)1; Zhao,SY(Zhao,Shuyu)1; Wu,JR(Wu,Jiarui)1; Wang,Qiyuan
2018
Source PublicationAtmospheric Chemistry and Physics
Volume18Issue:2018Pages:4639-4656
Subtype期刊论文
AbstractBlack carbon (BC) aerosol has important effects on the climate and hydrology of the Tibetan Plateau (TP). An intensive measurement campaign was conducted at Lulang (∼3300ma.s.l. – above sea level), southeastern TP, from September to October 2015, to investigate the sources and physicochemical characteristics of refractory BC (rBC) aerosol. The average rBC mass concentration was 0.31±0.55µgm−3, which is higher than most prior results for BC on the TP. A clear diurnal cycle in rBC showed high values in the morning and low values in the afternoon. A bivariate polar plot showed that rBC loadings varied with wind speed and direction, which also reflected the dominant transport direction. The estimated net surface rBC transport intensity was +0.05±0.29µgs−1m−2, indicating stronger transport from outside the TP compared with its interior. Cluster analysis and a concentration-weighted trajectory model connected emissions from north India to the high rBC loadings, but the effects of internal TP sources should not be overlooked. The average mass median diameter (MMD) of rBC was 160±23nm, with smaller MMDs on rainy days (145nm) compared with non-rainy days (164nm). The average number fraction of thickly coated rBC (FrBC) was 39±8%, and it increased with the O3 mixing ratios from 10:00 to 14:00LT, indicating that photochemical oxidation played a role in forming rBC coatings. The average rBC absorption enhancement (Eabs) was estimated to be 1.9, suggesting that light absorption by coated rBC particles was greater than for uncoated ones. The Eabs was strongly positively correlated with the FrBC, indicating an amplification of light absorption for internally mixed rBC. For rBC cores <170nm, Eabs was negatively correlated with MMD, but it was nearly constant for rBC cores > 170nm. Our study provides insight into the sources and evolution of rBC aerosol on the TP, and the results should be useful for improving models of the radiative effects of carbonaceous aerosols in this area.
DOI10.5194/acp-18-4639-2018
Indexed BySCI
Language英语
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Document Type期刊论文
Identifierhttp://ir.ieecas.cn/handle/361006/5361
Collection粉尘与环境研究室
Corresponding AuthorWang,Qiyuan
Affiliation1.Key Laboratory of Aerosol Chemistry and Physics, State Key Laboratory of Loess and Quaternary Geology,Institute of Earth Environment, Chinese Academy of Sciences, Xi’an, 710061, China
2.Institute of Global Environmental Change, Xi’an Jiaotong University, Xi’an, 710049, China
3.School of Human Settlements and Civil Engineering, Xi’an Jiaotong University, Xi’an, 710049, China
4.Department of Environmental Science and Engineering, School of Energy and Power Engineering, Xi’an JiaotongUniversity, Xi’an, 710049, China
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GB/T 7714
Wang,QY,Cao,JJ,Han,YM,et al. Sources and physicochemical characteristics of blackcarbon aerosol from the southeastern Tibetan Plateau:internal mixing enhances light absorption[J]. Atmospheric Chemistry and Physics,2018,18(2018):4639-4656.
APA Wang,QY.,Cao,JJ.,Han,YM.,Tian,J.,Zhu,CS.,...&Wang,Qiyuan.(2018).Sources and physicochemical characteristics of blackcarbon aerosol from the southeastern Tibetan Plateau:internal mixing enhances light absorption.Atmospheric Chemistry and Physics,18(2018),4639-4656.
MLA Wang,QY,et al."Sources and physicochemical characteristics of blackcarbon aerosol from the southeastern Tibetan Plateau:internal mixing enhances light absorption".Atmospheric Chemistry and Physics 18.2018(2018):4639-4656.
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