Personal exposure of PM2.5 emitted from solid fuels combustion forhousehold heating and cooking in rural Guanzhong Plain, northwesternChina

doi:10.1016/j.atmosenv.2018.05.018

IEECAS OpenIR > 粉尘与环境研究室

	Personal exposure of PM2.5 emitted from solid fuels combustion forhousehold heating and cooking in rural Guanzhong Plain, northwesternChina
	Xu,HM(Xu,Hongmei)1,2; Li,YQ(Li,Yaqi)1; Guinot, Benjamin 5; Wang,JH(Wang,Jinhui)6; He,KL(He,Kailai)1; Ho, K.F(Ho,Kai,Fai)7; Cao,JJ(Cao,Junji)3; Shen,ZX(Shen,Zhenxing)1; Sun,J(Sun,Jian)1; Lei,YL(Lei,Yali)1; Gong,XS(Gong,Xuesong)1,8; Zhang,T(Zhang,Ting)3; Xu,Hongmei
	2018-07
发表期刊	Atmospheric Environment
卷号	185 期号:2018 页码:196-206
文章类型	期刊论文
摘要	Household solid fuel combustion for heating and cooking in rural areas is an important source of fine particulate matter (PM2.5) in northwestern China, which largely contributes to PM2.5 personal exposure concentrations during the cold winter. There is a general lack of understanding about the personal exposure to PM2.5 and to its chemical components emitted from domestic solid fuel combustion in northwestern Chinese rural populations. In this work, personal exposure to PM2.5 was sampled using a portative device together with fixed indoor and outdoor fixed samplings in Guanzhong Plain in December 2016 for the purpose of characterizing personal exposure to PM2.5 as a function of different solid fuels used in rural households. The average housewife's personal exposure to PM2.5 concentration was 263.4 ± 105.8 μg m−3 (1σ, n = 30), which was about 40% higher than the values found indoors (186.5 ± 79.5 μg m−3, 1σ, n = 30) and outdoors (191.0 ± 85.3 μg m−3, 1σ, n = 30). High personal exposure PM2.5 levels were mainly related to the ignition of solid fuels for heating and cooking. Correlations among personal exposure, indoor and outdoor PM2.5 levels and their mutual ratios were computed to investigate how personal exposure to fine aerosols can be related to microenvironmental PM2.5 levels and to individual activities. The results showed that households using electric power for heating and cooking were characterized by an average personal exposure PM2.5 value of 156.8 ± 36.6 μg m−3 (1σ, n = 6) while personal exposure to PM2.5 in households using solid fuels was twice higher (310.8 ± 90.4 μg m−3, 1σ, n = 24). Solid fuel combustion products and related secondary formed species dominated PM2.5 mass in personal exposure, indoor and outdoor samples. Motor vehicle emission and various dust sources were two other main contributors identified. Our results demonstrated that the use of clean energy could be an effective measure to reduce personal exposure levels of PM2.5 emitted from domestic solid fuels combustion in winter in rural areas, which implied that the government should speed up the upgrade of the heating and cooking equipment fleet to protect the health of rural residents in northwestern China.
关键词	Personal Exposure Pm2.5 Solid Fuel Combustion Household Air Pollution Ambient Air Pollution
DOI	10.1016/j.atmosenv.2018.05.018
收录类别	SCI
所属项目编号	41503096 ; KHK1712 ; SKLLQG1722 ; 412413
语种	英语
项目资助者	Natural Science Foundation ofChina ; Natural Science Foundation ofChina ; Jiangsu Key Laboratory ofAtmospheric Environment Monitoring and Pollution Control ; Jiangsu Key Laboratory ofAtmospheric Environment Monitoring and Pollution Control ; State Key Laboratory of Loess andQuaternary Geology, Institute of Earth Environment, CAS ; State Key Laboratory of Loess andQuaternary Geology, Institute of Earth Environment, CAS ; Research Grants Council of the Hong Kong SpecialAdministrative Region of China ; Research Grants Council of the Hong Kong SpecialAdministrative Region of China
引用统计	被引频次：55[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.ieecas.cn/handle/361006/5333
专题	粉尘与环境研究室
通讯作者	Xu,Hongmei
作者单位	1.Department of Environmental Science and Engineering, Xi'an Jiaotong University, Xi'an, China 2.Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and PollutionControl (AEMPC), Nanjing University of Information Science & Technology, Nanjing, China 3.SKLLQG, Key Lab of Aerosol Chemistry & Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China 4.Health Science Center, Xi'an Jiaotong University, Xi'an, China 5.Laboratoire d’Aérologie, Université de Toulouse, CNRS, UPS, France 6.NICU, Xi'an Children's Hospital, Xi'an, China 7.JC School of Public Health and Primary Care, The Chinese University of Hong Kong, Hong Kong, China 8.Xi'an Polytechnic University, Xi'an, China
推荐引用方式 GB/T 7714	Xu,HM,Li,YQ,Guinot, Benjamin,et al. Personal exposure of PM2.5 emitted from solid fuels combustion forhousehold heating and cooking in rural Guanzhong Plain, northwesternChina[J]. Atmospheric Environment,2018,185(2018):196-206.
APA	Xu,HM.,Li,YQ.,Guinot, Benjamin.,Wang,JH.,He,KL.,...&Xu,Hongmei.(2018).Personal exposure of PM2.5 emitted from solid fuels combustion forhousehold heating and cooking in rural Guanzhong Plain, northwesternChina.Atmospheric Environment,185(2018),196-206.
MLA	Xu,HM,et al."Personal exposure of PM2.5 emitted from solid fuels combustion forhousehold heating and cooking in rural Guanzhong Plain, northwesternChina".Atmospheric Environment 185.2018(2018):196-206.

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