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Contributions of residential coal combustion to the air qualityin Beijing–Tianjin–Hebei (BTH), China: a case study
Li, X(Li, Xia)1,2; Wu, JR(Wu, Jiarui)1; Miriam Elser3; Feng, T(Feng, Tian)1; Cao, JJ(Cao, Junji)1; Imad El-Haddad3; Huang, RJ(Huang, Rujin)1; Tie, XX(Tie, Xuexi)1; André S. H. Prévôt3; Li, GH(Li, Guohui)1; Li, Guohui
2018-07-26
发表期刊Atmospheric Chemistry and Physics
卷号18期号:2018页码:10675-10691
文章类型期刊论文
其他摘要In the present study, the WRF-Chem model is used to assess contributions of residential coal combustion (RCC) emissions to the air quality in Beijing–Tianjin–Hebei (BTH) during a persistent air pollution episode from 9 to 25 January 2014. In general, the predicted temporal variations and spatial distributions of the mass concentrations of air pollutants are in good agreement with observations at monitoring sites in BTH. The WRF-Chem model also reasonably reproduces the temporal variations in aerosol species when compared with the aerosol mass spectrometer measurements in Beijing. The RCC emissions play an important role in the haze formation in BTH, contributing about 23.1% of PM2.5 (fine particulate matter) and 42.6% of SO2 during the simulation period on average. Organic aerosols dominate the PM2.5 from the RCC emissions in BTH, with a contribution of 42.8%, followed by sulfate (17.1%). The air quality in Beijing is remarkably improved when the RCC emissions in BTH and the surrounding areas are excluded in model simulations, with a 30% decrease in PM2.5 mass concentrations. However, if only the RCC emissions in Beijing are excluded, the local PM2.5 mass concentration is decreased by 18.0% on average. Our results suggest that the implementation of the residential coal replacement by clean energy sources in Beijing is beneficial to the local air quality. Should residential coal replacement be carried out in BTH and its surrounding areas, the air quality in Beijing would be improved remarkably. Further studies would need to consider uncertainties in the emission inventory and meteorological fields.
收录类别SCI
所属项目编号Quantitative Relationship and RegulationPrinciple between Regional Oxidation Capacity of Atmosphericand Air Quality, 2017YFC0210000 ; 41661144020
语种英语
项目资助者National Key R & D Plan ; National Key R & D Plan ; “Hundred Talents Program” of the Chinese Academy ofSciences and the National Natural Science Foundation of China ; “Hundred Talents Program” of the Chinese Academy ofSciences and the National Natural Science Foundation of China
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/5263
专题粉尘与环境研究室
通讯作者Li, Guohui
作者单位1.Key Lab of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences,Xi’an, China
2.University of Chinese Academy of Sciences, Beijing, China
3.Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen, Switzerland
推荐引用方式
GB/T 7714
Li, X(Li, Xia),Wu, JR(Wu, Jiarui),Miriam Elser,等. Contributions of residential coal combustion to the air qualityin Beijing–Tianjin–Hebei (BTH), China: a case study[J]. Atmospheric Chemistry and Physics,2018,18(2018):10675-10691.
APA Li, X.,Wu, JR.,Miriam Elser.,Feng, T.,Cao, JJ.,...&Li, Guohui.(2018).Contributions of residential coal combustion to the air qualityin Beijing–Tianjin–Hebei (BTH), China: a case study.Atmospheric Chemistry and Physics,18(2018),10675-10691.
MLA Li, X,et al."Contributions of residential coal combustion to the air qualityin Beijing–Tianjin–Hebei (BTH), China: a case study".Atmospheric Chemistry and Physics 18.2018(2018):10675-10691.
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