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Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion
Klein, Felix1; Pieber, Simone M.1; Ni, Haiyan2; Stefenelli, Giulia1; Bertrand, Amelie3; Kilic, Dogushan1; Pospisilova, Veronika1; Temime-Roussel, Brice3; Marchand, Nicolas3; El Haddad, Imad1; Slowik, Jay G.1; Baltensperger, Urs1; Cao, Junji2; Huang, Ru-Jin1,2; Prevot, Andre S. H.1
2018-03-06
发表期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
卷号52期号:5页码:2612-2617
文章类型Article
摘要Residential coal combustion is a significant contributor to particulate urban air pollution in Chinese mega cities and some regions in Europe. While the particulate emission factors and the chemical characteristics of the organic and inorganic aerosol from coal combustion have been extensively studied, the chemical composition and nonmethane organic gas (NMOG) emission factors from residential coal combustion are mostly unknown. We conducted 23 individual burns in a traditional Chinese stove used for heating and cooking using five different coals with Chinese origins, characterizing the NMOG emissions using a proton transfer reaction time-of-flight mass spectrometer. The measured emission factors range from 1.5 to 14.1 g/kg(coal) for bituminous coals and are below 0.1 g/kg(coal) A for anthracite coals. The emission factors from the bituminous coals are mostly influenced by the time until the coal is fully ignited. The emissions from the bituminous coals are dominated by aromatic and oxygenated aromatic compounds with a significant contribution of hydrocarbons. The results of this study can help to improve urban air pollution modeling in China and Eastern Europe and can be used to constrain a coal burning factor in ambient gas phase positive matrix factorization studies.
WOS标题词Science & Technology ; Technology ; Life Sciences & Biomedicine
DOI10.1021/acs.est.7b03960
关键词[WOS]HOUSEHOLD STOVES ; EMISSION FACTORS ; WOOD COMBUSTION ; HAZE EVENTS ; CHINA ; COOKSTOVES ; ATMOSPHERE ; POLLUTION ; CARBON ; PM2.5
收录类别SCI
语种英语
WOS研究方向Engineering ; Environmental Sciences & Ecology
WOS类目Engineering, Environmental ; Environmental Sciences
WOS记录号WOS:000427202700023
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文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/5226
专题粉尘与环境研究室
作者单位1.Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland
2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China
3.Aix Marseille Univ, CNRS, LCE, F-13331 Marseille, France
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Klein, Felix,Pieber, Simone M.,Ni, Haiyan,et al. Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2018,52(5):2612-2617.
APA Klein, Felix.,Pieber, Simone M..,Ni, Haiyan.,Stefenelli, Giulia.,Bertrand, Amelie.,...&Prevot, Andre S. H..(2018).Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion.ENVIRONMENTAL SCIENCE & TECHNOLOGY,52(5),2612-2617.
MLA Klein, Felix,et al."Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion".ENVIRONMENTAL SCIENCE & TECHNOLOGY 52.5(2018):2612-2617.
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