Enhanced light absorption due to the mixing state of black carbon in fresh biomass burning emissions | |
Wang, Qiyuan1; Cao, Junji1,2; Han, Yongming1,3; Tian, Jie4; Zhang, Yue4; Pongpiachan, Siwatt5; Zhang, Yonggang1; Li, Li1; Niu, Xinyi3; Shen, Zhenxing4; Zhao, Zhuzi1; Tipmanee, Danai6; Bunsomboonsakul, Suratta5; Chen, Yang7; Sun, Jian4 | |
2018-05-01 | |
发表期刊 | ATMOSPHERIC ENVIRONMENT |
卷号 | 180期号:5页码:184-191 |
文章类型 | Article |
摘要 | lack of information on the radiative effects of refractory black carbon (rBC) emitted from biomass burning is a significant gap in our understanding of climate change. A custom-made combustion chamber was used to simulate the open burning of crop residues and investigate the impacts of rBC size and mixing state on the particles' optical properties. Average rBC mass median diameters ranged from 141 to 162 nm for the rBC produced from different types of crop residues. The number fraction of thickly-coated rBC varied from 53 to 64%, suggesting that a majority of the freshly emitted rBC were internally mixed. By comparing the result of observed mass absorption cross-section to that calculated with Mie theory, large light absorption enhancement factors (1.7-1.9) were found for coated particles relative to uncoated cores. These effects were strongly positively correlated with the percentage of coated particles but independent of rBC core size. We suggest that rBC from open biomass burning may have strong impact on air pollution and radiative forcing immediately after their production. |
关键词 | Black Carbon Mixing State Size Distribution Light Absorption Biomass Burning |
WOS标题词 | Science & Technology ; Life Sciences & Biomedicine ; Physical Sciences |
DOI | 10.1016/j.atmosenv.2018.02.049 |
关键词[WOS] | QINGHAI-TIBETAN PLATEAU ; PHYSICAL-PROPERTIES ; CROSS-SECTION ; TRACE GASES ; SOUTH CHINA ; AEROSOL ; PARTICLES ; DEPENDENCE ; TRANSPORT ; CLIMATE |
收录类别 | SCI |
语种 | 英语 |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000430765300019 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ieecas.cn/handle/361006/5169 |
专题 | 粉尘与环境研究室 |
作者单位 | 1.Chinese Acad Sci, Key Lab Aerosol Chem & Phys, State Key Lab Loess & Quaternary Geol, Inst Earth Environm, Xian 710061, Shaanxi, Peoples R China 2.Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Shaanxi, Peoples R China 3.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Shaanxi, Peoples R China 4.Xi An Jiao Tong Univ, Sch Energy & Power Engn, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China 5.NIDA, Sch Social & Environm Dev, Bangkok 10240, Thailand 6.Prince Songkla Univ, Fac Technol & Environm, Phuket Campus, Phuket 83120, Thailand 7.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Qiyuan,Cao, Junji,Han, Yongming,et al. Enhanced light absorption due to the mixing state of black carbon in fresh biomass burning emissions[J]. ATMOSPHERIC ENVIRONMENT,2018,180(5):184-191. |
APA | Wang, Qiyuan.,Cao, Junji.,Han, Yongming.,Tian, Jie.,Zhang, Yue.,...&Sun, Jian.(2018).Enhanced light absorption due to the mixing state of black carbon in fresh biomass burning emissions.ATMOSPHERIC ENVIRONMENT,180(5),184-191. |
MLA | Wang, Qiyuan,et al."Enhanced light absorption due to the mixing state of black carbon in fresh biomass burning emissions".ATMOSPHERIC ENVIRONMENT 180.5(2018):184-191. |
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