| Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study | |
| Wu, Jiarui1,3; Bei, Naifang2; Li, Xia1,3; Cao, Junji1; Feng, Tian1; Wang, Yichen1; Tie, Xuexi1; Li, Guohui1 | |
| 2018-06-18 | |
| 发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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| 卷号 | 18期号:12页码:8491-8504 |
| 文章类型 | Article |
| 摘要 | During the Asian summer monsoon season, prevailing southeasterly-southwesterly winds are subject to delivering air pollutants from the North China Plain (NCP) to northeast and northwest China. In the present study, the WRF-CHEM model is used to evaluate contributions of trans-boundary transport of NCP emissions to the air quality in northeast and northwest China during a persistent air pollution episode from 22 to 28 May 2015. The WRF-CHEM model generally performs well in capturing the observed temporal variation and spatial distribution of fine particulate matter (PM2.5), ozone (O-3), and NO2. The simulated temporal variation of aerosol species is also in good agreement with measurements in Beijing during the episode. Model simulations show that NCP emissions contribute substantially to the PM2.5 level in Liaoning and Shanxi provinces, the adjacent downwind areas of the NCP, with an average of 24.2 and 13.9 mu g m(-3) during the episode, respectively. The PM2.5 contributions in Jilin and Shanxi provinces are also appreciable, with an average of 9.6 and 6.5 mu g m(-3), respectively. The average percentage contributions of NCP emissions to the PM2.5 level in Liaoning, Jilin, Shanxi, and Shaanxi provinces are 40.6, 27.5, 32.2, and 20.9 %, respectively. The NCP emissions contribute remarkably to the O-3 level in Liaoning province, with an average of 46.5 mu g m(-3), varying from 23.9 to 69.5 mu g m(-3). The O-3 level in Shanxi province is also influenced considerably by NCP emissions, with an average contribution of 35.1 mu g m(-3). The O-3 level in Shanxi province is also influenced considerably by NCP emissions, with an average contribution of 35.1 mu g m(-3). The average O-3 contributions of NCP emissions to Jilin and Shaanxi provinces are 28.7 and 20.7 mu g m(-3), respectively. The average percentage contributions of NCP emissions to the afternoon O-3 level in Liaoning, Jilin, Shanxi, and Shaanxi provinces are 27.4, 19.5, 21.2, and 15.8 %, respectively. However, the effect of NCP emissions on the air quality in Inner Mongolia is generally insignificant. Therefore, effective mitigation of NCP emissions not only improves the local air quality, but is also beneficial to the air quality in northeast and northwest China during the Asian summer monsoon season. |
| WOS标题词 | Science & Technology ; Physical Sciences |
| DOI | 10.5194/acp-18-8491-2018 |
| 关键词[WOS] | CAL-MEX 2010 ; METEOROLOGICAL UNCERTAINTIES ; MCMA-2006/MILAGRO CAMPAIGN ; AEROSOL CONCENTRATIONS ; SOURCE APPORTIONMENT ; FACTOR SEPARATION ; OZONE FORMATION ; FIELD CAMPAIGN ; HAZE FORMATION ; EASTERN CHINA |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| WOS类目 | Meteorology & Atmospheric Sciences |
| WOS记录号 | WOS:000435484300002 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.ieecas.cn/handle/361006/5094 |
| 专题 | 粉尘与环境研究室 |
| 通讯作者 | Li, Guohui |
| 作者单位 | 1.Chinese Acad Sci, Key Lab Aerosol Chem & Phys, SKLLQG, Inst Earth Environm, Xian, Shaanxi, Peoples R China 2.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Shaanxi, Peoples R China 3.Univ Chinese Acad Sci, Beijing, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wu, Jiarui,Bei, Naifang,Li, Xia,et al. Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(12):8491-8504. |
| APA | Wu, Jiarui.,Bei, Naifang.,Li, Xia.,Cao, Junji.,Feng, Tian.,...&Li, Guohui.(2018).Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(12),8491-8504. |
| MLA | Wu, Jiarui,et al."Widespread air pollutants of the North China Plain during the Asian summer monsoon season: a case study".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.12(2018):8491-8504. |
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| Widespread air pollu（23148KB） | 期刊论文 | 出版稿 | 开放获取 | CC BY-NC-SA | 请求全文 | |
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