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Carbonate weathering dominates magnesium isotopes in large rivers: Clues from the Yangtze River
Xu, Yang1,2; Jin, Zhangdong1,3; Gou, Long-Fei1; Galy, Albert4; Jin, Chenyang5; Chen, Chen1; Li, Chenzi1,2; Deng, Li1
通讯作者Jin, Zhangdong(zhdjin@ieecas.cn)
2022-01-20
发表期刊CHEMICAL GEOLOGY
ISSN0009-2541
卷号588页码:11
摘要Carbonate weathering regulates the short-term carbon (C) cycle and global climate due to its fast response to hydrological processes. The carbonate weathering flux needs to be well constrained to better understand the climate change at short time scale. Riverine magnesium (Mg) isotopes are sensitive to primary mineral dissolution and so have great potential to trace carbonate weathering. Global large rivers draining continental crust dominate weathering flux to the oceans, but how riverine Mg isotopes respond to carbonate weathering remains unclear. The Yangtze River drainage basin (YRDB) was selected to test the robustness of riverine Mg isotopes (delta Mg-26) in tracing continental carbonate weathering because it spans a wide range in lithology, geomorphology and climate. The riverine delta Mg-26 values within the YRDB show a decreasing trend from the headwater to the mainstream ranging from -1.36 parts per thousand to -0.59 parts per thousand The dissolved delta Mg-26 have strong negative correlations with carbonate weathering rate and intensity within the YRDB, indicating a sensitive response of riverine delta Mg-26 to the carbonate weathering flux. In a compilation of Mg fluxes and delta Mg-26 in the world's largest rivers, there is similar dominance of carbonate weathering on riverine Mg fluxes and isotopes. Therefore, we propose that riverine delta Mg-26 in large rivers are a robust tracer of carbonate weathering intensity. Intensifying carbonate weathering under global warming tends to increase riverine Mg and C fluxes to the oceans and thus the atmospheric CO2 sink at the millennial time scale.
关键词Carbonate weathering Mg isotopes Sr isotopes Weathering tracer The Yangtze River Global large rivers
DOI10.1016/j.chemgeo.2021.120677
关键词[WOS]MG ISOTOPES ; CHEMICAL-COMPOSITION ; CO2 CONSUMPTION ; TIBETAN-PLATEAU ; SILICATE ; FRACTIONATION ; GEOCHEMISTRY ; BASIN ; SR ; PRECIPITATION
收录类别SCI ; SCI
语种英语
资助项目NSFC[41991322] ; NSFC[41930864]
WOS研究方向Geochemistry & Geophysics
项目资助者NSFC
WOS类目Geochemistry & Geophysics
WOS记录号WOS:000731965800020
出版者ELSEVIER
引用统计
被引频次:15[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/17327
专题加速器质谱中心
通讯作者Jin, Zhangdong
作者单位1.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Xian 710061, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710049, Peoples R China
4.Univ Lorraine, Ctr Rech Petrograph & Geochim, CNRS, UMR7358, F-54500 Vandoeuvre Les Nancy, France
5.Tongji Univ, State Key Lab Marine Geol, Shanghai 200092, Peoples R China
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GB/T 7714
Xu, Yang,Jin, Zhangdong,Gou, Long-Fei,et al. Carbonate weathering dominates magnesium isotopes in large rivers: Clues from the Yangtze River[J]. CHEMICAL GEOLOGY,2022,588:11.
APA Xu, Yang.,Jin, Zhangdong.,Gou, Long-Fei.,Galy, Albert.,Jin, Chenyang.,...&Deng, Li.(2022).Carbonate weathering dominates magnesium isotopes in large rivers: Clues from the Yangtze River.CHEMICAL GEOLOGY,588,11.
MLA Xu, Yang,et al."Carbonate weathering dominates magnesium isotopes in large rivers: Clues from the Yangtze River".CHEMICAL GEOLOGY 588(2022):11.
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