| Stable carbon isotopic characteristics of fossil fuels in China | |
Wang, Peng1,2; Zhou, Weijian1,2,3,4; Xiong, Xiaohu1,2; Wu, Shugang1,2 ; Niu, Zhenchuan1,2,3; Cheng, Peng1,2; Du, Hua1,2; Hou, Yaoyao1,2
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| Corresponding Author | Zhou, Weijian(weijian@loess.llqg.ac.cn) |
| 2022-01-20 | |
| Source Publication | SCIENCE OF THE TOTAL ENVIRONMENT
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| ISSN | 0048-9697 |
| Volume | 805Pages:8 |
| Abstract | Good knowledge on the stable carbon isotopic composition (delta C-13) of fossil fuels is critical for the estimation of atmospheric CO2 sources. Here, we complied a comprehensive delta C-13 database including 336 coal, 580 oil, and 1160 natural gas data based on the extensive literature search, and conducted field measurements in two megacities, to characterize the delta C-13 signatures of Chinese fossil fuels. Results show that coal exhibits a narrow range and the most enriched in delta C-13 signature, oil displays intermediate variations both in the distribution and value of delta C-13. By contrast, natural gas is strongly depleted but became more enriched in delta C-13 signature due to the shift in production from isotopically light oil-type gas to isotopically heavy coal-type gas. We found an obvious overlap between the delta C-13 distributions of oil and natural gas, and the carbon isotopic difference between oil and natural gas is minimized in Ordos Basin. Therefore, we suggested that the geographic origin is a certain factor that must be considered when delta C-13 of fossil fuels is used to estimate CO2 source contributions, and the measurement of delta(CO2)-C-13 signatures of local end members is a better alternative in the absence of detailed information about the geographical origins of fossil fuels. This work is helpful in improving the ability to quantify CO2 sources of fossil fuel emissions in China, and also make a contribute to the global carbon isotope database. (C) 2021 Elsevier B.V. All rights reserved. |
| Keyword | Carbon isotope Fossil fuel Database End-member |
| DOI | 10.1016/j.scitotenv.2021.150240 |
| WOS Keyword | ATMOSPHERIC CO2 ; BIOGENIC GASES ; MIXING-RATIO ; EMISSIONS ; DELTA-C-13 ; DIOXIDE ; SPECTROSCOPY ; METHANE ; ANALYZER ; KRAKOW |
| Indexed By | SCI ; SCI |
| Language | 英语 |
| Funding Project | Strategic Priority Research Program of the Chinese Academy of Sciences[XDA23010302] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB40000000] ; National Natural Science Foundation of China[41730108] ; Natural Science Basic Research Program of Shaanxi Province[2021JQ-319] |
| WOS Research Area | Environmental Sciences & Ecology |
| Funding Organization | Strategic Priority Research Program of the Chinese Academy of Sciences ; National Natural Science Foundation of China ; Natural Science Basic Research Program of Shaanxi Province |
| WOS Subject | Environmental Sciences |
| WOS ID | WOS:000701667700015 |
| Publisher | ELSEVIER |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.ieecas.cn/handle/361006/17080 |
| Collection | 加速器质谱中心 第四纪科学与全球变化卓越创新中心 |
| Corresponding Author | Zhou, Weijian |
| Affiliation | 1.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Peoples R China 2.Xian AMS Ctr, Shaanxi Key Lab Accelerator Mass Spectrometry Tec, Xian 710061, Peoples R China 3.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Peoples R China 4.Xian Inst Innovat Earth Environm Res, Xian 710061, Peoples R China |
| Recommended Citation GB/T 7714 | Wang, Peng,Zhou, Weijian,Xiong, Xiaohu,et al. Stable carbon isotopic characteristics of fossil fuels in China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2022,805:8. |
| APA | Wang, Peng.,Zhou, Weijian.,Xiong, Xiaohu.,Wu, Shugang.,Niu, Zhenchuan.,...&Hou, Yaoyao.(2022).Stable carbon isotopic characteristics of fossil fuels in China.SCIENCE OF THE TOTAL ENVIRONMENT,805,8. |
| MLA | Wang, Peng,et al."Stable carbon isotopic characteristics of fossil fuels in China".SCIENCE OF THE TOTAL ENVIRONMENT 805(2022):8. |
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