Effects of Agricultural Waste Burning on PM2.5-Bound Polycyclic Aromatic Hydrocarbons, Carbonaceous Compositions, and Water-Soluble Ionic Species in the Ambient Air of Chiang-Mai, Thailand | |
ChooChuay, Chomsri1; Pongpiachan, Siwatt2; Tipmanee, Danai3; Deelaman, Woranuch1; Iadtem, Natthapong1; Suttinun, Oramas1; Wang, Qiyuan4,5; Xing, Li4,5; Li, Guohui4,5; Han, Yongming4,5; Hashmi, Muhammad Zaffar6; Palakun, Jittree7; Poshyachinda, Saran8; Aukkaravittayapun, Suparerk8; Surapipith, Vanisa8; Cao, Junji4,5 | |
通讯作者 | Pongpiachan, Siwatt(pongpiajun@gmail.com) |
2020-04-17 | |
发表期刊 | POLYCYCLIC AROMATIC COMPOUNDS |
ISSN | 1040-6638 |
页码 | 22 |
摘要 | PM2.5 is widely regarded as a major air pollutant due to its adverse health impacts and intimate relationship with the climate system. This study aims to characterize the chemical components (e.g., organic carbon (OC), elemental carbon (EC), water soluble ionic species (WSIS) and polycyclic aromatic hydrocarbons (PAHs) in PM2.5 collected at Doi-Inthanon in Chiang-Mai, Thailand, the highest mountain in Thailand. All samples (n = 50) were collected by MiniVolTM portable air samplers from March 2017 to March 2018. In this study we found the average PM2.5 concentration was 100 +/- 48.6 mu g m(-3). The OC/EC ratio was 6.8 +/- 3.0, and the decreasing order of the WSIS concentrations was SO42->Na+>Ca2+>NH4+>NO3->K+>Cl->NO2->Mg2+> F-. The total concentrations of nineteen PAHs were defined as the sum of Ace, Fl, Phe, Ant, Fluo, Pyr, B[a]A, Chry, B[b]F, B[k]F, B[a]F, B[e]P, B[a]P, Per, Ind, B[g,h,i]P, D[a,h]A, Cor, and D[a,e]P. The concentration of total PAHs was 2.361 +/- 2.154 mu g m(-3). Principal component analysis (PCA) highlights the importance of vehicular exhaust, biomass burning, diesel emissions, sea-salt aerosols and volatilization from fertilizers as the five dominant potential sources that accounted for 51.6%, 16.2%, 10.6%, 5.20% and 3.70% of the total variance, respectively. The rest of the 12.7% variance probably is associated with unidentified local and regional sources such as incinerators, joss paper/incense burning, and domestic cooking. Interestingly, the results from the source estimations from the PCA underlined the importance of vehicular exhaust as the major contributor to the PM2.5 concentrations in the ambient air of Don-Inthanon, Chiang-Mai province. However, it is crucial to emphasize that the impacts of agricultural waste burning, fossil fuel combustion, coal combustion and forest fires on the variations of OC, EC and WSIS contents were not negligible. |
关键词 | PM2 5 PAHs carbonaceous compositions water soluble ionic species biomass burning |
DOI | 10.1080/10406638.2020.1750436 |
关键词[WOS] | FINE PARTICULATE MATTER ; AEROSOL CHEMICAL PROFILE ; PORT THERMAL-DESORPTION ; NORTHERN INDO-CHINA ; SOURCE APPORTIONMENT ; ORGANIC-COMPOUNDS ; ATMOSPHERIC AEROSOLS ; ELEMENTAL CARBON ; SOURCE IDENTIFICATION ; POLLUTION SOURCES |
收录类别 | SCI ; SCI |
语种 | 英语 |
资助项目 | Institute of the Earth Environment, Chinese Academy of Science (IEECAS) ; Thailand Research Fund |
WOS研究方向 | Chemistry |
项目资助者 | Institute of the Earth Environment, Chinese Academy of Science (IEECAS) ; Thailand Research Fund |
WOS类目 | Chemistry, Organic |
WOS记录号 | WOS:000527656900001 |
出版者 | TAYLOR & FRANCIS LTD |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ieecas.cn/handle/361006/14737 |
专题 | 粉尘与环境研究室 |
通讯作者 | Pongpiachan, Siwatt |
作者单位 | 1.Prince Songkla Univ, Fac Environm Management, Hat Yai Campus, Hat Yai, Thailand 2.Natl Inst Dev Adm, Ctr Res & Dev Disaster Prevent & Management, Sch Social & Environm Dev, 118 Moo 3,Sereethai Rd, Bangkok 10240, Thailand 3.Prince Songkla Univ Phuket, Fac Technol & Environm, Phuket, Thailand 4.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Xian, Peoples R China 5.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian, Peoples R China 6.OMSATS Univ, Dept Meteorol, Islamabad, Pakistan 7.Royal Patronage VRU, Valaya Alongkorn Rajabhat Univ, Fac Educ, Pathum Thani, Thailand 8.Natl Astron Res Inst Thailand, Publ Org, Chiang Mai, Thailand |
推荐引用方式 GB/T 7714 | ChooChuay, Chomsri,Pongpiachan, Siwatt,Tipmanee, Danai,et al. Effects of Agricultural Waste Burning on PM2.5-Bound Polycyclic Aromatic Hydrocarbons, Carbonaceous Compositions, and Water-Soluble Ionic Species in the Ambient Air of Chiang-Mai, Thailand[J]. POLYCYCLIC AROMATIC COMPOUNDS,2020:22. |
APA | ChooChuay, Chomsri.,Pongpiachan, Siwatt.,Tipmanee, Danai.,Deelaman, Woranuch.,Iadtem, Natthapong.,...&Cao, Junji.(2020).Effects of Agricultural Waste Burning on PM2.5-Bound Polycyclic Aromatic Hydrocarbons, Carbonaceous Compositions, and Water-Soluble Ionic Species in the Ambient Air of Chiang-Mai, Thailand.POLYCYCLIC AROMATIC COMPOUNDS,22. |
MLA | ChooChuay, Chomsri,et al."Effects of Agricultural Waste Burning on PM2.5-Bound Polycyclic Aromatic Hydrocarbons, Carbonaceous Compositions, and Water-Soluble Ionic Species in the Ambient Air of Chiang-Mai, Thailand".POLYCYCLIC AROMATIC COMPOUNDS (2020):22. |
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