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High-resolution simulation of wintertime fossil fuel CO2 in Beijing, China: Characteristics, sources, and regional transport
Feng, Tian1,2; Zhou, Weijian1,2; Wu, Shugang1,2; Niu, Zhenchuan1,2; Cheng, Peng1,2; Xiong, Xiaohu1,2; Li, Guohui1,3
通讯作者Zhou, Weijian(weijian@loess.llqg.ac.cn)
2019-02-01
发表期刊ATMOSPHERIC ENVIRONMENT
ISSN1352-2310
卷号198页码:226-235
摘要In this study, a high-resolution simulation of fossil fuel CO2 in Beijing and surrounding areas, China, during January 2014 is performed to investigate the characteristics and sources of Beijing fossil fuel CO2 (FFCO2) mixing ratios and the impact of regional transport. The model reasonably reproduces the observed meteorological fields in the study domain, including temperature, relative humidity, wind speed, and wind direction. The simulated CO2 and CO mixing ratios in Beijing are in good agreement with the measurements. Elevated FFCO2 levels are produced by the model in megacities, such as Beijing, Tianjin, Shijiazhuang, and Baoding. The model result shows that FFCO2 mixing ratios are significantly correlated with observed total CO2, CO, and PM2.5 concentrations in Beijing. Sensitivity experiments show that Beijing FFCO2 is mainly from industry and residential emissions (35% for each), followed by power plant (21%) and transportation (9%) emissions in January 2014. Spatially, the largest contributor for Beijing FFCO2 is the local source, and regional transport also plays an important role in winter. The impact of regional transport is associated with wind direction, in which south/east (north/west) wind tends to accumulate (dilute) Beijing FFCO2. In addition, the roles of regional transport during haze and clean episodes are significantly distinct in winter, and more contribution is found in haze episodes.
关键词Fossil fuel CO2 Regional transport P-2.5 WRF-Chem
DOI10.1016/j.atmosenv.2018.10.054
关键词[WOS]CARBON-DIOXIDE ; METEOROLOGICAL UNCERTAINTIES ; ISOTOPIC COMPOSITION ; EMISSION INVENTORY ; ENERGY-CONSUMPTION ; MODELING SYSTEM ; HEAVY HAZE ; ATMOSPHERE ; (CO2)-C-14 ; EUROPE
收录类别SCI ; SCI
语种英语
资助项目China Postdoctoral Science Foundation[2017M613236] ; National Natural Science Foundation of China[41730108] ; Bureau of Major R&D Programs, Chinese Academy of Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
项目资助者China Postdoctoral Science Foundation ; National Natural Science Foundation of China ; Bureau of Major R&D Programs, Chinese Academy of Sciences
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000455693900022
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:6[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/14384
专题粉尘与环境研究室
通讯作者Zhou, Weijian
作者单位1.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
2.Xian AMS Ctr, Xian 710061, Shaanxi, Peoples R China
3.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China
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Feng, Tian,Zhou, Weijian,Wu, Shugang,et al. High-resolution simulation of wintertime fossil fuel CO2 in Beijing, China: Characteristics, sources, and regional transport[J]. ATMOSPHERIC ENVIRONMENT,2019,198:226-235.
APA Feng, Tian.,Zhou, Weijian.,Wu, Shugang.,Niu, Zhenchuan.,Cheng, Peng.,...&Li, Guohui.(2019).High-resolution simulation of wintertime fossil fuel CO2 in Beijing, China: Characteristics, sources, and regional transport.ATMOSPHERIC ENVIRONMENT,198,226-235.
MLA Feng, Tian,et al."High-resolution simulation of wintertime fossil fuel CO2 in Beijing, China: Characteristics, sources, and regional transport".ATMOSPHERIC ENVIRONMENT 198(2019):226-235.
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