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Increased secondary aerosol contribution and possible processing on polluted winter days in China
Wang, Yichen1,2; Chen, Ji3; Wang, Qiyuan2,4; Qin, Quande1; Ye, Jianhuai5; Han, Yuemei2; Li, Li1; Zhen, Wei1; Zhi, Qiang6; Zhang, Yixuan2; Cao, Junji2,4
2019-06-01
发表期刊ENVIRONMENT INTERNATIONAL
ISSN0160-4120
卷号127页码:78-84
摘要

China experiences severe particulate pollution, especially in winter, and determining the characteristics of particulate matter (PM) during pollution events is imperative for understanding the sources and causes of the pollution. However, inconsistencies have been found in the aerosol composition, sources and secondary processing among reported studies. Modern meta-analysis was used to probe the PM chemical characteristics and processing in winter at four representative regions of China, and the first finding was that secondary aerosol formation was the major effect factor for PM pollution. The secondary inorganic species behaved differently in the four regions: sulfate, nitrate, and ammonium increased in the Beijing-Tianjin-Hebei (BTH) and Guanzhong (GZ) areas, but only nitrate increased in the Pearl River Delta (PRD) and Yangtze River Delta (YRD) regions. The increased production of secondary organic aerosol (SOA) was probably caused by aqueous-phase processing in the GZ and BTH regions and by photochemical reactions in the PRD. Finally, we suggest future AMS/ACSM observations should focus on the aerosol characteristics in rural areas in winter in China.

关键词Secondary aerosols Aqueous-phase reactions Photochemical reactions Polluted days Winter
DOI10.1016/j.envint.2019.03.021
关键词[WOS]ATMOSPHERIC SUBMICRON AEROSOLS ; PM2.5 CHEMICAL-COMPOSITION ; REAL-TIME CHARACTERIZATION ; FINE PARTICULATE MATTER ; HUMIC-LIKE SUBSTANCES ; SOURCE APPORTIONMENT ; ORGANIC AEROSOLS ; AIR-QUALITY ; PARTICLE COMPOSITION ; MASS-SPECTROMETRY
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[71804115] ; National Natural Science Foundation of China[21661132005] ; Open Fund of the State Key Laboratory of Loess and Quaternary Geology[SKLLQG1834] ; China Postdoctoral Science Foundation[2018M640809] ; Key Research and Development Program of Shaanxi Province ; Youth Innovation Promotion Association CAS
WOS研究方向Environmental Sciences & Ecology
项目资助者National Natural Science Foundation of China ; Open Fund of the State Key Laboratory of Loess and Quaternary Geology ; China Postdoctoral Science Foundation ; Key Research and Development Program of Shaanxi Province ; Youth Innovation Promotion Association CAS
WOS类目Environmental Sciences
WOS记录号WOS:000467383500008
出版者PERGAMON-ELSEVIER SCIENCE LTD
引用统计
被引频次:51[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/13886
专题粉尘与环境研究室
第四纪科学与全球变化卓越创新中心
通讯作者Wang, Qiyuan; Qin, Quande; Cao, Junji
作者单位1.Shenzhen Univ, Coll Management, Shenzhen 518060, Peoples R China
2.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, SKLLQG, Xian, Shaanxi, Peoples R China
3.Aarhus Univ, Ctr Circular Bioecon, Dept Agroecol, BlichersAlle 20, DK-8830 Tjele, Denmark
4.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
5.Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
6.Cent Univ Finance & Econ, Sch Govt Adm, Beijing, Peoples R China
推荐引用方式
GB/T 7714
Wang, Yichen,Chen, Ji,Wang, Qiyuan,et al. Increased secondary aerosol contribution and possible processing on polluted winter days in China[J]. ENVIRONMENT INTERNATIONAL,2019,127:78-84.
APA Wang, Yichen.,Chen, Ji.,Wang, Qiyuan.,Qin, Quande.,Ye, Jianhuai.,...&Cao, Junji.(2019).Increased secondary aerosol contribution and possible processing on polluted winter days in China.ENVIRONMENT INTERNATIONAL,127,78-84.
MLA Wang, Yichen,et al."Increased secondary aerosol contribution and possible processing on polluted winter days in China".ENVIRONMENT INTERNATIONAL 127(2019):78-84.
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