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Characteristics of wintertime VOCs in suburban and urban Beijing: concentrations, emission ratios, and festival effects
Li, Kun1,2,3; Li, Junling1,2; Tong, Shengrui1,2; Wang, Weigang1,2; Huang, Ru-Jin4; Ge, Maofa1,2,5
通讯作者Ge, Maofa(gemaofa@iccas.ac.cn)
2019-06-19
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
卷号19期号:12页码:8021-8036
摘要Measurements of volatile organic compounds (VOCs) were performed at a suburban site and an urban site in Beijing during the winter of 2014-2015. The VOC concentrations and emission ratios (ERs) to CO were compared at these two sites. It is found that though the VOC concentrations at the urban site are 2.67 +/- 1.15 times of those at the suburban site, the ERs are similar (within a factor of 1.5). It is indicated that (1) the VOCs at suburban areas are mainly from the transportation from the urban areas and (2) the ERs measured at the urban areas are also valid for the surrounding suburban areas. By comparing the diurnal variations and the contribution of anthropogenic emissions at both sites, we find that the photochemical processes are very active at the urban site, and these processes play an important role in the daytime oxygenated VOC (OVOC) formation. The methanol at the urban site and the formic acid at the suburban site probably have additional sources, which are attributed to be solvent use and soil/agriculture, respectively. The festival effects from the Chinese New Year (CNY) were investigated. The VOC concentrations decreased similar to 60 % during CNY holidays, probably due to the population migration during festival holidays. In addition, fireworks are found to be an important source of acetonitrile, aromatics, and some OVOCs during the CNY festival and should be controlled more strictly. This study provides key characteristics of wintertime VOCs in suburban and urban Beijing and has implications for better understanding the atmospheric chemistry of VOCs in and around this megacity.
DOI10.5194/acp-19-8021-2019
关键词[WOS]VOLATILE ORGANIC-COMPOUNDS ; SECONDARY SOURCES ; AEROSOL COMPOSITION ; FINE PARTICULATE ; MIXING RATIOS ; HAZE EVENTS ; MEXICO-CITY ; PTR-MS ; FIREWORKS ; PHASE
收录类别SCI ; SCI
语种英语
资助项目National Key Research and Development Program of China[2016YFC0202202] ; National Key Research and Development Program of China[2017YFC0212701] ; National Natural Science Foundation of China[91544227] ; National Natural Science Foundation of China[21477134] ; National Natural Science Foundation of China[91644219]
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
项目资助者National Key Research and Development Program of China ; National Natural Science Foundation of China
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS记录号WOS:000472156200001
出版者COPERNICUS GESELLSCHAFT MBH
引用统计
被引频次:52[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/13816
专题粉尘与环境研究室
通讯作者Ge, Maofa
作者单位1.Chinese Acad Sci, BNLMS, State Key Lab Struct Chem Unstable & Stable Speci, CAS Res Educ Ctr Excellence Mol Sci,Inst Chem, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Sch Chem Sci, Beijing 100049, Peoples R China
3.Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
5.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Fujian, Peoples R China
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GB/T 7714
Li, Kun,Li, Junling,Tong, Shengrui,et al. Characteristics of wintertime VOCs in suburban and urban Beijing: concentrations, emission ratios, and festival effects[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(12):8021-8036.
APA Li, Kun,Li, Junling,Tong, Shengrui,Wang, Weigang,Huang, Ru-Jin,&Ge, Maofa.(2019).Characteristics of wintertime VOCs in suburban and urban Beijing: concentrations, emission ratios, and festival effects.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(12),8021-8036.
MLA Li, Kun,et al."Characteristics of wintertime VOCs in suburban and urban Beijing: concentrations, emission ratios, and festival effects".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.12(2019):8021-8036.
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