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Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts
Chang, Tian1,2,3; Lu, Jiaqi1; Shen, Zhenxing1,3; Zhang, Bin1; Huang, Yu3; Cao, Junji3; Liu, Hongxia1; Veerapandian, Savita K. P.2; De Geyter, Nathalie2; Morent, Rino2
Corresponding AuthorShen, Zhenxing(zxshen@mail.xjtu.edu.cn)
2019-08-14
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN0888-5885
Volume58Issue:32Pages:14719-14728
AbstractA system combining nonthermal plasma (NTP) and catalysis using Mn-Co/HZSM-5 catalyst has been developed to promote the oxidation of acetaldehyde and reduce the production of ozone. The introduction of catalyst improved the oxidation of acetaldehyde and inhibited the generation of O-3 in comparison with the NTP alone system. The mixed MnCo/HZSM-5 catalyst demonstrated the highest catalytic activity among the various prepared catalysts, and this was ascribed to its crystalline structure, redox property, and adsorbed surface oxygen of the catalyst. The removal efficiency of acetaldehyde and COx yield were positively associated with the specific energy density (SED), and they were inversely related to the gas flow rate. Nevertheless, the energy yield was in negative correlation with the SED and in positive association with the gas flow rate. Moreover, the impact of different catalysts on the acceleration of acetaldehyde degradation in the hybrid system was discussed by developing a simple kinetic model.
DOI10.1021/acs.iecr.9b02668
WOS KeywordMIXED OXIDES ; OXIDATION ; TOLUENE ; MN ; GAS ; DECOMPOSITION ; COMBUSTION ; PRODUCTS ; DEGRADATION ; SYSTEM
Indexed BySCI ; SCI
Language英语
Funding Projectproject DepollutAir of Interreg V France-Wallonie-Vlaanderen ; National Science Foundation of China (NSFC)[41573138] ; State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, CAS[SKLLQG1616] ; China Scholarship Council (CSC)[201806280087] ; Hundred Talent Program of the Chinese Academy of Sciences
WOS Research AreaEngineering
Funding Organizationproject DepollutAir of Interreg V France-Wallonie-Vlaanderen ; National Science Foundation of China (NSFC) ; State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, CAS ; China Scholarship Council (CSC) ; Hundred Talent Program of the Chinese Academy of Sciences
WOS SubjectEngineering, Chemical
WOS IDWOS:000481568600013
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:10[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ieecas.cn/handle/361006/13599
Collection粉尘与环境研究室
Corresponding AuthorShen, Zhenxing
Affiliation1.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China
2.Univ Ghent, Res Unit Plasma Technol, Dept Appl Phys, Fac Engn & Architecture, Sint Pietersnieuwstr 41-B4, B-9000 Ghent, Belgium
3.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, SKLLQG, Xian 710049, Shaanxi, Peoples R China
Recommended Citation
GB/T 7714
Chang, Tian,Lu, Jiaqi,Shen, Zhenxing,et al. Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2019,58(32):14719-14728.
APA Chang, Tian.,Lu, Jiaqi.,Shen, Zhenxing.,Zhang, Bin.,Huang, Yu.,...&Morent, Rino.(2019).Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,58(32),14719-14728.
MLA Chang, Tian,et al."Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 58.32(2019):14719-14728.
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