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Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts
Chang, Tian1,2,3; Lu, Jiaqi1; Shen, Zhenxing1,3; Zhang, Bin1; Huang, Yu3; Cao, Junji3; Liu, Hongxia1; Veerapandian, Savita K. P.2; De Geyter, Nathalie2; Morent, Rino2
通讯作者Shen, Zhenxing(zxshen@mail.xjtu.edu.cn)
2019-08-14
发表期刊INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN0888-5885
卷号58期号:32页码:14719-14728
摘要A system combining nonthermal plasma (NTP) and catalysis using Mn-Co/HZSM-5 catalyst has been developed to promote the oxidation of acetaldehyde and reduce the production of ozone. The introduction of catalyst improved the oxidation of acetaldehyde and inhibited the generation of O-3 in comparison with the NTP alone system. The mixed MnCo/HZSM-5 catalyst demonstrated the highest catalytic activity among the various prepared catalysts, and this was ascribed to its crystalline structure, redox property, and adsorbed surface oxygen of the catalyst. The removal efficiency of acetaldehyde and COx yield were positively associated with the specific energy density (SED), and they were inversely related to the gas flow rate. Nevertheless, the energy yield was in negative correlation with the SED and in positive association with the gas flow rate. Moreover, the impact of different catalysts on the acceleration of acetaldehyde degradation in the hybrid system was discussed by developing a simple kinetic model.
DOI10.1021/acs.iecr.9b02668
关键词[WOS]MIXED OXIDES ; OXIDATION ; TOLUENE ; MN ; GAS ; DECOMPOSITION ; COMBUSTION ; PRODUCTS ; DEGRADATION ; SYSTEM
收录类别SCI ; SCI
语种英语
资助项目project DepollutAir of Interreg V France-Wallonie-Vlaanderen ; National Science Foundation of China (NSFC)[41573138] ; State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, CAS[SKLLQG1616] ; China Scholarship Council (CSC)[201806280087] ; Hundred Talent Program of the Chinese Academy of Sciences
WOS研究方向Engineering
项目资助者project DepollutAir of Interreg V France-Wallonie-Vlaanderen ; National Science Foundation of China (NSFC) ; State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, CAS ; China Scholarship Council (CSC) ; Hundred Talent Program of the Chinese Academy of Sciences
WOS类目Engineering, Chemical
WOS记录号WOS:000481568600013
出版者AMER CHEMICAL SOC
引用统计
被引频次:20[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/13599
专题粉尘与环境研究室
通讯作者Shen, Zhenxing
作者单位1.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China
2.Univ Ghent, Res Unit Plasma Technol, Dept Appl Phys, Fac Engn & Architecture, Sint Pietersnieuwstr 41-B4, B-9000 Ghent, Belgium
3.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, SKLLQG, Xian 710049, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Chang, Tian,Lu, Jiaqi,Shen, Zhenxing,et al. Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2019,58(32):14719-14728.
APA Chang, Tian.,Lu, Jiaqi.,Shen, Zhenxing.,Zhang, Bin.,Huang, Yu.,...&Morent, Rino.(2019).Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,58(32),14719-14728.
MLA Chang, Tian,et al."Post Plasma Catalysis for the Removal of Acetaldehyde Using Mn-Co/HZSM-5 Catalysts".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 58.32(2019):14719-14728.
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