The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China
Wang, Xudong1,2,3; Liu, Guijian1,2; Zhou, Chuncai1,2
通讯作者Liu, Guijian(lgj@ustc.edu.cn)
2019-08-28
发表期刊ENVIRONMENTAL FORENSICS
ISSN1527-5922
页码10
摘要The trace elements (TEs) in coal are of great concern due to their toxicity and bioavailability. The coal, bottom ash, fly ash and gaseous species were sampled to study the partitioning and environmental behaviors of TEs during coal combustion. The mineral and phase characterizations of coal combustion residue were determined by X-ray powder diffraction (XRD) and fourier transform infrared spectroscopy (FTIR), respectively. The gaseous emission, risk assessment code and leaching experiment EN 12457 Part 2 procedure were employed to assess the potential environmental impacts. The concentrations of TEs in all the collected samples were determined by inductively coupled plasma mass spectrometry (ICP-MS). During combustion, the mineral compositions of coal (kaolinite, quartz, illite, pyrite and calcite) were changed to mullite, quartz, hematite, lime, magnetite and anhydrite. Arsenic, Cd, Cu, Pb and Zn were emitted mainly in fly ash and gaseous phases. In the current unconfined deposits, the TEs (As, Cu, Pb and Zn) in bottom ash and fly ash may pose a medium risk to the environment. High regularization and management countermeasures including immobilization/stabilization, re-utilization of combustion ash, and controlled disposal should be conducted to eliminate/minimize environmental and ecological risks in coal activities areas.
关键词Coal combustion trace elements partition behavior environmental impacts
DOI10.1080/15275922.2019.1657984
关键词[WOS]CHEMICAL-COMPOSITION ; FLY ASHES ; MULTICOMPONENT UTILIZATION ; FEED COALS ; COMBUSTION ; FATE ; METALS ; MATTER ; VOLATILITY ; MINERALOGY
收录类别SCI ; SCI
语种英语
资助项目National Basic Research Program of China (973 Program)[2016YFC0201600] ; National Natural Science Foundation of China[41702166] ; National Natural Science Foundation of China[41672144] ; Anhui Provincial Natural Science Foundation[1708085QE110] ; National Postdoctoral Program for Innovative Talents[BX201700222] ; China Postdoctoral Science Foundation[2017M622011]
WOS研究方向Environmental Sciences & Ecology
项目资助者National Basic Research Program of China (973 Program) ; National Natural Science Foundation of China ; Anhui Provincial Natural Science Foundation ; National Postdoctoral Program for Innovative Talents ; China Postdoctoral Science Foundation
WOS类目Environmental Sciences
WOS记录号WOS:000484135700001
出版者TAYLOR & FRANCIS LTD
引用统计
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/13513
专题黄土与第四纪地质国家重点实验室(2010~)
通讯作者Liu, Guijian
作者单位1.Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China
2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Shaanxi, Peoples R China
3.Anhui Publ Welf Geol Survey Management Ctr, Dept Nat Resources Anhui Prov, Hefei, Anhui, Peoples R China
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Wang, Xudong,Liu, Guijian,Zhou, Chuncai. The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China[J]. ENVIRONMENTAL FORENSICS,2019:10.
APA Wang, Xudong,Liu, Guijian,&Zhou, Chuncai.(2019).The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China.ENVIRONMENTAL FORENSICS,10.
MLA Wang, Xudong,et al."The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China".ENVIRONMENTAL FORENSICS (2019):10.
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