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Exploring the impact of chemical composition on aerosol light extinction during winter in a heavily polluted urban area of China
Zhou, Yaqing1,2,3; Wang, Qiyuan1,2,3,4; Zhang, Xu5; Wang, Yichen6; Liu, Suixin1,2,4; Wang, Meng1,2,3; Tian, Jie1,2,4; Zhu, Chongshu1,2,4; Huang, Rujin1,2,4; Zhang, Qian7; Zhang, Ting1,2,4; Zhou, Jiamao1,2,4; Dai, Wenting1,2,4; Cao, Junji1,2,4
Corresponding AuthorWang, Qiyuan(wangqy@ieecas.cn) ; Cao, Junji(cao@loess.llqg.ac.cn)
2019-10-01
Source PublicationJOURNAL OF ENVIRONMENTAL MANAGEMENT
ISSN0301-4797
Volume247Pages:766-775
AbstractAn intensive measurement campaign was conducted in Xi'an, China from December 2012-January 2013 to investigate the chemical composition, formation, and optical properties of PM1. The PM1 mass concentration (average = 138.8 +/- 83.2 mu g m(-3)) accounted for similar to 50% of the PM2.5 mass. Organic aerosols (OA) and secondary inorganic aerosols (SIA) were the most abundant PM1 components, contributing 53.0% and 35.0% to the mass, respectively. Both primary emissions and aqueous-phase oxidation of secondary aerosols played roles in the pollution episodes. The average light scattering and absorption coefficients during the campaign were 805 +/- 581 Mm(-1) and 123 +/- 96 Mm(-1), respectively. Both the mass scattering and mass absorption efficiencies for PM1 were higher than that for PM2.5.1, indicating stronger ability of light extinction for the smaller particles at visible wavelengths compared with the larger ones. The contributions of aerosol species to light extinction coefficients under two visibility conditions were estimated based on multiple linear regression models, and the OA was found to be the largest contributor to light extinction in both cases. A larger contribution of SIA to light extinction for visibility < 5 km demonstrated its greater impacts on visibility during heavy pollution conditions. These findings provide insights into the importance of submicron particles for pollution and visibility degradation in northwestern China.
KeywordPM1 Aerosol species Pollution formation mechanisms Optical properties
DOI10.1016/j.jenvman.2019.06.100
WOS KeywordBLACK CARBON AEROSOL ; OPTICAL-PROPERTIES ; SOURCE APPORTIONMENT ; ORGANIC AEROSOLS ; FINE PARTICLES ; BOUNDARY-LAYER ; AIR-POLLUTION ; BROWN CARBON ; MIXING STATE ; HAZE EVENTS
Indexed BySCI ; SCI
Language英语
Funding ProjectNational Natural Science Foundation of China[21661132005] ; Key Research and Development Program of Shaanxi Province[2018ZDCXL-SF-30-5] ; National Key Research and Development Program - Ministry of Science & Technology of China[2017YFC0212200] ; Youth Innovation Promotion Association, Chinese Academy of Sciences[2019402]
WOS Research AreaEnvironmental Sciences & Ecology
Funding OrganizationNational Natural Science Foundation of China ; Key Research and Development Program of Shaanxi Province ; National Key Research and Development Program - Ministry of Science & Technology of China ; Youth Innovation Promotion Association, Chinese Academy of Sciences
WOS SubjectEnvironmental Sciences
WOS IDWOS:000483635000077
PublisherACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD
Citation statistics
Cited Times:8[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ieecas.cn/handle/361006/13399
Collection粉尘与环境研究室
第四纪科学与全球变化卓越创新中心
Corresponding AuthorWang, Qiyuan; Cao, Junji
Affiliation1.Chinese Acad Sci, State Key Lab Loess & Quaternary Geol, Inst Earth Environm, Xian 710061, Shaanxi, Peoples R China
2.Chinese Acad Sci, Key Lab Aerosol Chem & Phys, Inst Earth Environm, Xian 710061, Shaanxi, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
5.Xian Environm Monitor Stn, Xian 710100, Shaanxi, Peoples R China
6.Shenzhen Univ, Coll Management, Shenzhen 518060, Peoples R China
7.Xian Univ Architecture & Technol, Sch Environm & Municipal Engn, Xian 710055, Shaanxi, Peoples R China
Recommended Citation
GB/T 7714
Zhou, Yaqing,Wang, Qiyuan,Zhang, Xu,et al. Exploring the impact of chemical composition on aerosol light extinction during winter in a heavily polluted urban area of China[J]. JOURNAL OF ENVIRONMENTAL MANAGEMENT,2019,247:766-775.
APA Zhou, Yaqing.,Wang, Qiyuan.,Zhang, Xu.,Wang, Yichen.,Liu, Suixin.,...&Cao, Junji.(2019).Exploring the impact of chemical composition on aerosol light extinction during winter in a heavily polluted urban area of China.JOURNAL OF ENVIRONMENTAL MANAGEMENT,247,766-775.
MLA Zhou, Yaqing,et al."Exploring the impact of chemical composition on aerosol light extinction during winter in a heavily polluted urban area of China".JOURNAL OF ENVIRONMENTAL MANAGEMENT 247(2019):766-775.
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