Emission Characteristics of Primary Brown Carbon Absorption From Biomass and Coal Burning: Development of an Optical Emission Inventory for China | |
Tian, J (Tian, Jie); Wang, QY (Wang, Qiyuan); Ni, HY (Ni, Haiyan); Wang, M (Wang, Meng); Zhou, YQ (Zhou, Yaqing); Han, YM (Han, Yongming); Shen, ZX (Shen, Zhenxing); Pongpiachan, S (Pongpiachan, Siwatt); Zhang, NN (Zhang, Ningning); Zhao, ZZ (Zhao, Zhuzi); Zhang, Q (Zhang, Qian); Zhang, Y (Zhang, Yue); Long, X (Long, Xin); Cao, JJ (Cao, Junji) | |
通讯作者 | Wang, Qiyuan(wangqy@ieecas.cn) ; Shen, Zhenxing(zxshen@mail.xjtu.edu.cn) ; Cao, Junji(cao@loess.llqg.ac.cn) |
2019-02-16 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
ISSN | 2169-897X |
卷号 | 124期号:3页码:1879-1893 |
产权排序 | 2 |
摘要 | Brown carbon (BrC) affects the Earth's radiative balance due to its strong light absorption at short wavelengths. A custom-made combustion chamber was used to simulate biomass and coal burning and to investigate the emission characteristics of BrC absorption. Absorption angstrom ngstrom exponents (AAEs) at the wavelength pair of 370 and 880nm ranged from 1.19 to 3.25, suggesting the possible existence of BrC in biomass- and coal-burning emissions. Based on the assumption that AAE(BC)=1.0, BrC from biomass burning contributed to 41-85% of the total particles light absorption at 370nm, which is much higher than that from coal burning (15-18%). The estimated absorption emission factors of BrC at 370nm for biomass and coal burning were 15-47 and 2-13m(2)/kg, respectively. A 10x10km gridded BrC optical emission inventory for biomass and coal burning in China for 2015 was developed based on the measured absorption emission factors of BrC values and high-resolution activity data. The total annual BrC absorption cross section emissions from biomass and residential coal burning were 4,194Gm(2) (relative uncertainty at the 95% confidence level of -33.2, 41.2%) and 615Gm(2) (-39.3, 40.1%), respectively. These results should be useful for improving estimates of the radiative effects of BrC in China. |
DOI | 10.1029/2018JD029352 |
关键词[WOS] | SOLUBLE ORGANIC-CARBON ; ANGSTROM EXPONENT AAE ; LIGHT-ABSORPTION ; BLACK CARBON ; PARTICULATE MATTER ; WAVELENGTH DEPENDENCE ; SPECTRAL DEPENDENCE ; AEROSOL EMISSIONS ; COMBUSTION ; MASS |
收录类别 | SCI ; SCIE |
语种 | 英语 |
资助项目 | Ministry of Science and Technology of the People's Republic China[2013FY112700] ; National Natural Science Foundation of China[41503118] ; National Natural Science Foundation of China[41661144020] ; National Natural Science Foundation of China[41673125] ; National Natural Science Foundation of China[41705106] ; China Postdoctoral Science Foundation[2015M580890] ; China Postdoctoral Science Foundation[2018M633523] |
WOS研究方向 | Meteorology & Atmospheric Sciences |
项目资助者 | Ministry of Science and Technology of the People's Republic China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000459377000039 |
出版者 | AMER GEOPHYSICAL UNION |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ieecas.cn/handle/361006/10963 |
专题 | 粉尘与环境研究室 |
通讯作者 | Wang, QY (Wang, Qiyuan); Shen, ZX (Shen, Zhenxing); Cao, JJ (Cao, Junji) |
作者单位 | 1.Xi An Jiao Tong Univ, Sch Energy & Power Engn, Dept Environm Sci & Engn, Xian, Shaanxi, Peoples R China 2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Key Lab Aerosol Chem & Phys, Xian, Shaanxi, Peoples R China 3.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Shaanxi, Peoples R China 4.NIDA, Sch Social & Environm Dev, Bangkok, Thailand 5.Xi An Jiao Tong Univ, Inst Global Environm Change, Xian, Shaanxi, Peoples R China |
推荐引用方式 GB/T 7714 | Tian, J ,Wang, QY ,Ni, HY ,et al. Emission Characteristics of Primary Brown Carbon Absorption From Biomass and Coal Burning: Development of an Optical Emission Inventory for China[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2019,124(3):1879-1893. |
APA | Tian, J .,Wang, QY .,Ni, HY .,Wang, M .,Zhou, YQ .,...&Cao, JJ .(2019).Emission Characteristics of Primary Brown Carbon Absorption From Biomass and Coal Burning: Development of an Optical Emission Inventory for China.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,124(3),1879-1893. |
MLA | Tian, J ,et al."Emission Characteristics of Primary Brown Carbon Absorption From Biomass and Coal Burning: Development of an Optical Emission Inventory for China".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 124.3(2019):1879-1893. |
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