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Effects of biomass briquetting and carbonization on PM2.5 emission from residential burning in Guanzhong Plain, China
Sun, J (Sun, Jian)1,2; Shen, ZX (Shen, Zhenxing)2; Zhang, Y (Zhang, Yue)2; Zhang, Q (Zhang, Qian)2; Wang, FR (Wang, Furong)3; Wang, T (Wang, Tao)3; Chang, XJ (Chang, Xiaojian)3; Lei, YL (Lei, Yali)2; Xu, HM (Xu, Hongmei)2; Cao, JJ (Cao, Junji)4; Zhang, NN (Zhang, Ningning)4; Liu, SX (Liu, Suixin)4; Li, XX (Li, Xuxiang)1
2019-05-15
发表期刊FUEL
卷号244页码:379-387
产权排序4
摘要In this study, maize straw, wheat straw, and wood branches and their processed products (i.e., briquettes and charcoals) were used to investigate the emission factors (EFs) of PM2.5 components and the influence of form changing. The EFs of organic carbon (OC) was 241 +/- 39.7 to 3920 +/- 792 mg kg(-1); OC was the largest contributor in PM2.5. The EFs of PM2.5, OC and elemental carbon (EC) demonstrated that charcoal was the most efficient in reducing PM2.5 and carbonaceous fraction emissions, followed by briquettes compared with raw fuels in residential burning use. Among cations, K+ had the highest EF, whereas Cl- has the highest EF among anions; the presence of both K+ and Cl- was attributable to high abundance in biomass. Cl, K, S, and Na (in descending order) contributed more than 95% of total elements with high EFs; the other elements, particularly heavy metals, had very low EFs. The EFs of total polycyclic aromatic hydrocarbons (PAHs) and saccharides were in the following order of magnitude: raw fuels > briquettes > charcoals. PAHs with four rings (i.e., pyrenes) dominated the total PAHs in PM2.5-, whereas among saccharides, levoglucosan had the largest EFs (0.03-110.41 mg kg(-1)). Briquettes, with simple process and reasonable cost, demonstrated a good ability in decreasing PM2.5 emission with potential of 53% (765,000-427,000 t year(-1)), and their emission reduction potential were much higher for straws than for branches. Charcoals demonstrated considerable emission reduction potential for straw (93.7% averagely for PM2.5 and compositions) and comparable for wood branches (80% averagely) while its complex process and high cost should be considered. More than 600,000 t of PM2.5 and thousands of tons of PAHs and saccharides are estimated to be eliminated annually if all raw biomass fuels are processed through carbonization. Considering the efficiency-cost ratios, biomass briquetting may aid clean heating in rural areas, in addition to the "natural gas and electricity replacement strategy," in China and other countries facing similar problems.
关键词Emission factors Biomass Fuel processing Form changing Emission reduction
收录类别SCI ; SCIE
语种英语
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/10958
专题粉尘与环境研究室
作者单位1.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian 710049, Shaanxi, Peoples R China;
2.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Shaanxi, Peoples R China;
3.Agr Technol & Extens Cent Xian City, Xian, Shaanxi, Peoples R China;
4.Chinese Acad Sci, Key Lab Aerosol Chem & Phys, Inst Earth Environm, Xian 710049, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Sun, J ,Shen, ZX ,Zhang, Y ,et al. Effects of biomass briquetting and carbonization on PM2.5 emission from residential burning in Guanzhong Plain, China[J]. FUEL,2019,244:379-387.
APA Sun, J .,Shen, ZX .,Zhang, Y .,Zhang, Q .,Wang, FR .,...&Li, XX .(2019).Effects of biomass briquetting and carbonization on PM2.5 emission from residential burning in Guanzhong Plain, China.FUEL,244,379-387.
MLA Sun, J ,et al."Effects of biomass briquetting and carbonization on PM2.5 emission from residential burning in Guanzhong Plain, China".FUEL 244(2019):379-387.
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