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Molecular composition and size distribution of sugars, sugar-alcohols and carboxylic acids in airborne particles during a severe urban haze event caused by wheat straw burning
Wang, GH (Wang, Gehui)[1,2,4]; Chen, CL (Chen, Chunlei)[1]; Li, JJ (Li, Jianjun)[1]; Zhou, BH (Zhou, Bianhong)[1]; Xie, MJ (Xie, Mingjie)[3]; Hu, SY (Hu, Shuyuan)[3]; Kawamura, K (Kawamura, Kimitaka)[2]; Chen, Y (Chen, Yan)[4]
2011-05-30
发表期刊ATMOSPHERIC ENVIRONMENT
卷号45期号:15页码:2473-2479
文章类型期刊论文
摘要

Molecular compositions and size distributions of water-soluble organic compounds (WSOC, i.e., sugars, sugar-alcohols and carboxylic acids) in particles from urban air of Nanjing, China during a severe haze event caused by field burning of wheat straw were characterized and compared with those in the summer and autumn non-haze periods. During the haze event levoglucosan (4030 ng m(-3)) was the most abundant compound among the measured WSOC, followed by succinic acid, malic acid, glycerol, arabitol and glucose, being different from those in the non-haze samples, in which sucrose or azelaic acid showed a second highest concentration, although levoglucosan was the highest. The measured WSOC in the haze event were 2-20 times more than those in the non-hazy days. Size distribution results showed that there was no significant change in the compound peaks in coarse mode (>2.1 mu m) with respect to the haze and non-haze samples, but a large difference in the fine fraction (<2.1 mu m) was found with a sharp increase during the hazy days mostly due to the increased emissions of wheat straw burning. Molecular compositions of organic compounds in the fresh smoke particles from wheat straw burning demonstrate that sharply increased concentrations of glycerol and succinic and malic acids in the fine particles during the haze event were mainly derived from the field burning of wheat straw, although the sources of glucose and related sugar-alcohols whose concentrations significantly increased in the fine haze samples are unclear. Compared to that in the fresh smoke particles of wheat straw burning an increase in relative abundance of succinic acid to levoglucosan during the haze event suggests a significant production of secondary organic aerosols during transport of the smoke plumes.

关键词Water-soluble organic compounds Biomass burning Atmospheric aerosols Composition and size distribution Levoglucosan and succinic acid
DOI10.1016/j.atmosenv.2011.02.045
收录类别SCI
语种英语
引用统计
被引频次:99[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/10269
专题粉尘与环境研究室
通讯作者Wang, GH (Wang, Gehui)[1,2,4]
作者单位1.State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710075, China;
2.Institute of Low Temperature Science, Hokkaido University, Sapporo 060-0819, Japan;
3.School of the Environment, Nanjing University, Nanjing 210093, China;
4.School of Human Settlement and Civil Engineering, Xi’an Jiaotong University, Xi’an 710049, China
推荐引用方式
GB/T 7714
Wang, GH ,Chen, CL ,Li, JJ ,et al. Molecular composition and size distribution of sugars, sugar-alcohols and carboxylic acids in airborne particles during a severe urban haze event caused by wheat straw burning[J]. ATMOSPHERIC ENVIRONMENT,2011,45(15):2473-2479.
APA Wang, GH .,Chen, CL .,Li, JJ .,Zhou, BH .,Xie, MJ .,...&Chen, Y .(2011).Molecular composition and size distribution of sugars, sugar-alcohols and carboxylic acids in airborne particles during a severe urban haze event caused by wheat straw burning.ATMOSPHERIC ENVIRONMENT,45(15),2473-2479.
MLA Wang, GH ,et al."Molecular composition and size distribution of sugars, sugar-alcohols and carboxylic acids in airborne particles during a severe urban haze event caused by wheat straw burning".ATMOSPHERIC ENVIRONMENT 45.15(2011):2473-2479.
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