Observation of atmospheric aerosols at Mt. Hua and Mt. Tai in central and east China during spring 2009-Part 1: EC, OC and inorganic ions | |
Wang, G (Wang, G.)[1,2]; Li, J (Li, J.)[2]; Cheng, C (Cheng, C.)[1]; Hu, S (Hu, S.)[3]; Xie, M (Xie, M.)[3]; Gao, S (Gao, S.)[3]; Zhou, B (Zhou, B.)[4]; Dai, W (Dai, W.)[1]; Cao, J (Cao, J.)[1]; An, Z (An, Z.)[1] | |
2011 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
卷号 | 11期号:9页码:4221-4235 |
文章类型 | 期刊论文 |
摘要 | PM(10) and size-segregated samples were simultaneously collected at Mt. Hua (2060 ma.s.l.) and Mt. Tai (1545 ma.s.l.) in central and east coastal China during spring, 2009 including an intensive dust storm event occurring on 24 April, and determined for EC, OC and inorganic ions. During the non-dust storm period particles, EC, OC and ions except for SO(4)(2-) were 2-10 times more abundant at Mt. Tai than at Mt. Hua. SO(4)(2-) (13 +/- 7.1 mu g m(-3)) at Mt. Hua was the dominant ion, followed by NO(3)(-) (5.0 +/- 3.9 mu g m(-3)), NH(4)(+) (2.5 +/- 1.3 mu g m(-3)) and Ca(2+) (1.6 +/- 0.8 mu g m(-3)). In contrast, at Mt. Tai NO(3)(-) was most abundant (20 +/- 14 mu g m(-3)), followed by SO(4)(2-) (16 +/- 13 mu g m(-3)), NH(4)(+) (12 +/- 8.9 mu g m(-3)) and Ca(2+) (3.9 +/- 2.1 mu g m(-3)). The fact of NO(3)(-) exceeding over SO(4)(2-) at Mt. Tai may suggest the changes in chemical composition of the atmosphere over east China due to sharply increasing vehicle emission. pH values of the water-extracts of PM(10) samples indicate that at the two mountain sites aerosols transported from the south regions are more acidic than those from the north and more acidic at Mt. Tai than at Mt. Hua during the non-dust storm period. During the dust storm event particle mass, OC, Na(+), K(+), Mg(2+) and Ca(2+) at both sites increased by a factor of 1-9, while EC, NO(3)(-) and NH(4)(+) decreased by 20-80 %. However, SO(4)(2-) concentrations (13 +/- 7.7 mu g m(-3) at Mt. Hua and 15 +/- 5.6 mu g m(-3) at Mt. Tai, respectively) at the two sites during the episode were comparable and did not change significantly compared to those in the non-dust storm period, probably due to a similar level of free tropospheric SO(2) in central and east China. |
DOI | 10.5194/acp-11-4221-2011 |
收录类别 | SCI |
语种 | 英语 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ieecas.cn/handle/361006/10268 |
专题 | 粉尘与环境研究室 |
通讯作者 | Wang, G (Wang, G.)[1,2] |
作者单位 | 1.State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences,Xi’an 710075, China; 2.Department of Environmental Science and Engineering, Xi’an Jiaotong University, Xi’an 710049, China; 3.School of the Environment, State Key Laboratory of Pollution Control and Resources Reuse, Nanjing University,Nanjing 210093, China; 4.Department of Geographical Science and Environment Engineering, Baoji University of Art and Science,Baoji 721013, China |
推荐引用方式 GB/T 7714 | Wang, G ,Li, J ,Cheng, C ,et al. Observation of atmospheric aerosols at Mt. Hua and Mt. Tai in central and east China during spring 2009-Part 1: EC, OC and inorganic ions[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2011,11(9):4221-4235. |
APA | Wang, G .,Li, J .,Cheng, C .,Hu, S .,Xie, M .,...&An, Z .(2011).Observation of atmospheric aerosols at Mt. Hua and Mt. Tai in central and east China during spring 2009-Part 1: EC, OC and inorganic ions.ATMOSPHERIC CHEMISTRY AND PHYSICS,11(9),4221-4235. |
MLA | Wang, G ,et al."Observation of atmospheric aerosols at Mt. Hua and Mt. Tai in central and east China during spring 2009-Part 1: EC, OC and inorganic ions".ATMOSPHERIC CHEMISTRY AND PHYSICS 11.9(2011):4221-4235. |
条目包含的文件 | ||||||
文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | ||
Observation of atmos(12445KB) | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | 请求全文 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论