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Long-Term Trends in Visibility and at Chengdu, China
Wang, QY (Wang, Qiyuan)[ 1,2 ]; Cao, JJ (Cao, Junji)[ 2,3 ]; Tao, J (Tao, Jun)[ 4 ]; Li, N (Li, Nan)[ 2 ]; Su, XO (Su, Xiaoli)[ 2 ]; Chen, LWA (Chen, L. W. Antony)[ 5 ]; Wang, P (Wang, Ping)[ 2 ]; Shen, ZX (Shen, Zhenxing)[ 1 ]; Liu, SX (Liu, Suixin)[ 2 ]; Dai, WT (Dai, Wenting)[ 2 ]
2013-07-18
发表期刊PLOS ONE
卷号8期号:7页码:e68894
文章类型期刊论文
摘要

Long-term (1973 to 2010) trends in visibility at Chengdu, China were investigated using meteorological data from the U.S. National Climatic Data Center. The visual range exhibited a declining trend before 1982, a slight increase between 1983 and 1995, a sharp decrease between 1996 and 2005, and some improvements after 2006. The trends in visibility were generally consistent with the economic development and implementation of pollution controls in China. Intensive PM2.5 measurements were conducted from 2009 to 2010 to determine the causes of visibility degradation. An analysis based on a modification of the IMPROVE approach indicated that PM2.5 ammonium bisulfate contributed 27.7% to the light extinction coefficient (bext); this was followed by organic mass (21.7%), moisture (20.6%), and ammonium nitrate (16.3%). Contributions from elemental carbon (9.4%) and soil dust (4.3%) were relatively minor. Anthropogenic aerosol components (sulfate, nitrate, and elemental carbon) and moisture at the surface also were important determinants of the aerosol optical depth (AOD) at 550 nm, and the spatial distributions of both bext and AOD were strongly affected by regional topography. A Positive Matrix Factorization receptor model suggested that coal combustion was the largest contributor to PM2.5 mass (42.3%) and the dry-air light-scattering coefficient (47.7%); this was followed by vehicular emissions (23.4% and 20.5%, respectively), industrial emissions (14.9% and 18.8%), biomass burning (12.8% and 11.9%), and fugitive dust (6.6% and 1.1%). Our observations provide a scientific basis for improving visibility in this area.

DOI10.1371/journal.pone.0068894
收录类别SCI
语种英语
引用统计
被引频次:19[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/10007
专题粉尘与环境研究室
通讯作者Cao, JJ (Cao, Junji)[ 2,3 ]
作者单位1.Department of Environmental Science and Engineering, Xi’an Jiaotong University, Xi’an, China;
2.Key Lab of Aerosol Science & Technology, SKLLQG, Institute of EarthEnvironment, Chinese Academy of Sciences, Xi’an, China;
3.Institute of Global Environmental Change, Xi’an Jiaotong University, Xi’an, China;
4.South China Institute ofEnvironmental Sciences, SEPA, Guangzhou, China;
5.Division of Atmospheric Sciences, Desert Research Institute, Reno, Nevada, United States of America
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GB/T 7714
Wang, QY ,Cao, JJ ,Tao, J ,et al. Long-Term Trends in Visibility and at Chengdu, China[J]. PLOS ONE,2013,8(7):e68894.
APA Wang, QY .,Cao, JJ .,Tao, J .,Li, N .,Su, XO .,...&Dai, WT .(2013).Long-Term Trends in Visibility and at Chengdu, China.PLOS ONE,8(7),e68894.
MLA Wang, QY ,et al."Long-Term Trends in Visibility and at Chengdu, China".PLOS ONE 8.7(2013):e68894.
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